Valence tautomerism of singly protonated 9-aminoacridine and its implications for intercalative interactions with nucleic acids

Electronic absorption and fluorescence spectroscopy were used to show that the singly protonated 9-aminoacridine cation exists as the vinylogous cyclic amidine valence tautomer, the 9-iminoacridan monocation, in ground and excited states when in aqueous solution at physiological pH. The evidence ind...

وصف كامل

محفوظ في:
التفاصيل البيبلوغرافية
المؤلف الرئيسي: Capomacchia, Anthony C. (author)
مؤلفون آخرون: Casper, Jay (author), Schulman, Stephen G. (author)
التنسيق: article
منشور في: 1974
الوصول للمادة أونلاين:http://hdl.handle.net/10725/6334
http://dx.doi.org/10.1002/jps.2600630823
http://libraries.lau.edu.lb/research/laur/terms-of-use/articles.php
http://onlinelibrary.wiley.com/doi/10.1002/jps.2600630823/full
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الوصف
الملخص:Electronic absorption and fluorescence spectroscopy were used to show that the singly protonated 9-aminoacridine cation exists as the vinylogous cyclic amidine valence tautomer, the 9-iminoacridan monocation, in ground and excited states when in aqueous solution at physiological pH. The evidence indicates that the 9-aminoacridine monocation may intercalate into double-helical DNA in an orientation different from that employed by other acridine derivatives.