Purification of colloidal oil in water emulsions by cationic adsorbent prepared from recycled polyethylene waste

<p>This study deals with removing crude oil droplets from colloidal oil in water emulsions. The target was the development of efficient adsorbents for the tertiary treatment of industrial-produced water (PW). The novel adsorbent was designed from recycled low-density polyethylene (LDPE) powder...

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محفوظ في:
التفاصيل البيبلوغرافية
المؤلف الرئيسي: Sarah Hailan (17787584) (author)
مؤلفون آخرون: Priya Ghosh (1814422) (author), Patrik Sobolciak (9166184) (author), Peter Kasak (1360617) (author), Anton Popelka (2804842) (author), Mabrouk Ouederni (14153478) (author), Samer Adham (9182153) (author), Mohamed Chehimi (2645980) (author), Gordon McKay (1755814) (author), Igor Krupa (1389267) (author)
منشور في: 2024
الموضوعات:
الوسوم: إضافة وسم
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author Sarah Hailan (17787584)
author2 Priya Ghosh (1814422)
Patrik Sobolciak (9166184)
Peter Kasak (1360617)
Anton Popelka (2804842)
Mabrouk Ouederni (14153478)
Samer Adham (9182153)
Mohamed Chehimi (2645980)
Gordon McKay (1755814)
Igor Krupa (1389267)
author2_role author
author
author
author
author
author
author
author
author
author_facet Sarah Hailan (17787584)
Priya Ghosh (1814422)
Patrik Sobolciak (9166184)
Peter Kasak (1360617)
Anton Popelka (2804842)
Mabrouk Ouederni (14153478)
Samer Adham (9182153)
Mohamed Chehimi (2645980)
Gordon McKay (1755814)
Igor Krupa (1389267)
author_role author
dc.creator.none.fl_str_mv Sarah Hailan (17787584)
Priya Ghosh (1814422)
Patrik Sobolciak (9166184)
Peter Kasak (1360617)
Anton Popelka (2804842)
Mabrouk Ouederni (14153478)
Samer Adham (9182153)
Mohamed Chehimi (2645980)
Gordon McKay (1755814)
Igor Krupa (1389267)
dc.date.none.fl_str_mv 2024-01-25T15:00:00Z
dc.identifier.none.fl_str_mv 10.1016/j.psep.2024.01.042
dc.relation.none.fl_str_mv https://figshare.com/articles/journal_contribution/Purification_of_colloidal_oil_in_water_emulsions_by_cationic_adsorbent_prepared_from_recycled_polyethylene_waste/26490964
dc.rights.none.fl_str_mv CC BY 4.0
info:eu-repo/semantics/openAccess
dc.subject.none.fl_str_mv Engineering
Environmental engineering
Materials engineering
Environmental sciences
Environmental biotechnology
Polyethylene
Adsorption
Emulsions
Crude oil
Produced water
Tertiary treatment
dc.title.none.fl_str_mv Purification of colloidal oil in water emulsions by cationic adsorbent prepared from recycled polyethylene waste
dc.type.none.fl_str_mv Text
Journal contribution
info:eu-repo/semantics/publishedVersion
text
contribution to journal
description <p>This study deals with removing crude oil droplets from colloidal oil in water emulsions. The target was the development of efficient adsorbents for the tertiary treatment of industrial-produced water (PW). The novel adsorbent was designed from recycled low-density polyethylene (LDPE) powder grafted by the cationic polymer. The cationic polymer was synthesized directly on the LDPE surface by plasma-induced radical polymerization. A positively charged adsorbent was chosen due to the negative character of oily droplets to enhance separation efficiency in treating oil-water emulsions. The separation was performed in both batch and filtration modes. Absorption/adsorption uptake capacities showed a sigmoidal S-shape that was analyzed using the Sips model and compared with the newly developed empirical model. Both models showed a remarkable coincidence in the description of experimental data. The separation efficiency of the novel adsorbent was also tested in a filtration mode mimicking a commonly used deep-bed filtration technology. The comparison of the separation efficiency for various sorbents indicated a supreme performance of novel adsorbent. This study demonstrates the potential of a relatively cheap, prepared commodity-based adsorbent for the purification of emulsified oily polluted water in both batch and filtration configurations. This study also contributes to the recycling of polyethylene waste because LDPE attracts meager interest in recycled LLDPE due to many obstacles to reusing LDPE waste for its reprocessing as packaging materials.</p><h2>Other Information</h2> <p> Published in: Process Safety and Environmental Protection<br> License: <a href="http://creativecommons.org/licenses/by/4.0/" target="_blank">http://creativecommons.org/licenses/by/4.0/</a><br>See article on publisher's website: <a href="https://dx.doi.org/10.1016/j.psep.2024.01.042" target="_blank">https://dx.doi.org/10.1016/j.psep.2024.01.042</a></p>
eu_rights_str_mv openAccess
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identifier_str_mv 10.1016/j.psep.2024.01.042
network_acronym_str Manara2
network_name_str Manara2
oai_identifier_str oai:figshare.com:article/26490964
publishDate 2024
repository.mail.fl_str_mv
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rights_invalid_str_mv CC BY 4.0
spelling Purification of colloidal oil in water emulsions by cationic adsorbent prepared from recycled polyethylene wasteSarah Hailan (17787584)Priya Ghosh (1814422)Patrik Sobolciak (9166184)Peter Kasak (1360617)Anton Popelka (2804842)Mabrouk Ouederni (14153478)Samer Adham (9182153)Mohamed Chehimi (2645980)Gordon McKay (1755814)Igor Krupa (1389267)EngineeringEnvironmental engineeringMaterials engineeringEnvironmental sciencesEnvironmental biotechnologyPolyethyleneAdsorptionEmulsionsCrude oilProduced waterTertiary treatment<p>This study deals with removing crude oil droplets from colloidal oil in water emulsions. The target was the development of efficient adsorbents for the tertiary treatment of industrial-produced water (PW). The novel adsorbent was designed from recycled low-density polyethylene (LDPE) powder grafted by the cationic polymer. The cationic polymer was synthesized directly on the LDPE surface by plasma-induced radical polymerization. A positively charged adsorbent was chosen due to the negative character of oily droplets to enhance separation efficiency in treating oil-water emulsions. The separation was performed in both batch and filtration modes. Absorption/adsorption uptake capacities showed a sigmoidal S-shape that was analyzed using the Sips model and compared with the newly developed empirical model. Both models showed a remarkable coincidence in the description of experimental data. The separation efficiency of the novel adsorbent was also tested in a filtration mode mimicking a commonly used deep-bed filtration technology. The comparison of the separation efficiency for various sorbents indicated a supreme performance of novel adsorbent. This study demonstrates the potential of a relatively cheap, prepared commodity-based adsorbent for the purification of emulsified oily polluted water in both batch and filtration configurations. This study also contributes to the recycling of polyethylene waste because LDPE attracts meager interest in recycled LLDPE due to many obstacles to reusing LDPE waste for its reprocessing as packaging materials.</p><h2>Other Information</h2> <p> Published in: Process Safety and Environmental Protection<br> License: <a href="http://creativecommons.org/licenses/by/4.0/" target="_blank">http://creativecommons.org/licenses/by/4.0/</a><br>See article on publisher's website: <a href="https://dx.doi.org/10.1016/j.psep.2024.01.042" target="_blank">https://dx.doi.org/10.1016/j.psep.2024.01.042</a></p>2024-01-25T15:00:00ZTextJournal contributioninfo:eu-repo/semantics/publishedVersiontextcontribution to journal10.1016/j.psep.2024.01.042https://figshare.com/articles/journal_contribution/Purification_of_colloidal_oil_in_water_emulsions_by_cationic_adsorbent_prepared_from_recycled_polyethylene_waste/26490964CC BY 4.0info:eu-repo/semantics/openAccessoai:figshare.com:article/264909642024-01-25T15:00:00Z
spellingShingle Purification of colloidal oil in water emulsions by cationic adsorbent prepared from recycled polyethylene waste
Sarah Hailan (17787584)
Engineering
Environmental engineering
Materials engineering
Environmental sciences
Environmental biotechnology
Polyethylene
Adsorption
Emulsions
Crude oil
Produced water
Tertiary treatment
status_str publishedVersion
title Purification of colloidal oil in water emulsions by cationic adsorbent prepared from recycled polyethylene waste
title_full Purification of colloidal oil in water emulsions by cationic adsorbent prepared from recycled polyethylene waste
title_fullStr Purification of colloidal oil in water emulsions by cationic adsorbent prepared from recycled polyethylene waste
title_full_unstemmed Purification of colloidal oil in water emulsions by cationic adsorbent prepared from recycled polyethylene waste
title_short Purification of colloidal oil in water emulsions by cationic adsorbent prepared from recycled polyethylene waste
title_sort Purification of colloidal oil in water emulsions by cationic adsorbent prepared from recycled polyethylene waste
topic Engineering
Environmental engineering
Materials engineering
Environmental sciences
Environmental biotechnology
Polyethylene
Adsorption
Emulsions
Crude oil
Produced water
Tertiary treatment