New insights into the impact of graphene oxide characteristics on foam stability: from bulk behavior to bubble dynamics

<p>Foam stability is critical for various engineering applications. Despite this, foam generated from pure surfactant solutions is often highly unstable, limiting its practical effectiveness. In this study, we investigate the potential of graphene oxide (GO) as an aqueous foam stabilizer under...

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Main Author: Ali U. Chaudhry (19724362) (author)
Other Authors: Ahmed Abdala (5743205) (author), Rizwan Muneer (19724365) (author), Muhammad Rehan Hashmet (19724368) (author), Thomas Deniel Seers (22631147) (author), Nayef Alyafei (19862553) (author), Reza Sadr (14158884) (author), Harris Sajjad Rabbani (14489205) (author)
Published: 2025
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author Ali U. Chaudhry (19724362)
author2 Ahmed Abdala (5743205)
Rizwan Muneer (19724365)
Muhammad Rehan Hashmet (19724368)
Thomas Deniel Seers (22631147)
Nayef Alyafei (19862553)
Reza Sadr (14158884)
Harris Sajjad Rabbani (14489205)
author2_role author
author
author
author
author
author
author
author_facet Ali U. Chaudhry (19724362)
Ahmed Abdala (5743205)
Rizwan Muneer (19724365)
Muhammad Rehan Hashmet (19724368)
Thomas Deniel Seers (22631147)
Nayef Alyafei (19862553)
Reza Sadr (14158884)
Harris Sajjad Rabbani (14489205)
author_role author
dc.creator.none.fl_str_mv Ali U. Chaudhry (19724362)
Ahmed Abdala (5743205)
Rizwan Muneer (19724365)
Muhammad Rehan Hashmet (19724368)
Thomas Deniel Seers (22631147)
Nayef Alyafei (19862553)
Reza Sadr (14158884)
Harris Sajjad Rabbani (14489205)
dc.date.none.fl_str_mv 2025-11-10T15:00:00Z
dc.identifier.none.fl_str_mv 10.1016/j.molliq.2025.128848
dc.relation.none.fl_str_mv https://figshare.com/articles/journal_contribution/New_insights_into_the_impact_of_graphene_oxide_characteristics_on_foam_stability_from_bulk_behavior_to_bubble_dynamics/30636161
dc.rights.none.fl_str_mv CC BY 4.0
info:eu-repo/semantics/openAccess
dc.subject.none.fl_str_mv Engineering
Chemical engineering
Materials engineering
Nanotechnology
Foam stability
Nanoparticles
Bubble dynamics
Nano-graphene oxide
dc.title.none.fl_str_mv New insights into the impact of graphene oxide characteristics on foam stability: from bulk behavior to bubble dynamics
dc.type.none.fl_str_mv Text
Journal contribution
info:eu-repo/semantics/publishedVersion
text
contribution to journal
description <p>Foam stability is critical for various engineering applications. Despite this, foam generated from pure surfactant solutions is often highly unstable, limiting its practical effectiveness. In this study, we investigate the potential of graphene oxide (GO) as an aqueous foam stabilizer under highly saline conditions, using bulk- and bubble-scale experiments. Previous studies have shown that GO, at very low concentrations (∼300 ppm), can negatively impact foam stability, highlighting the importance of surface modification to enhance its performance as a foam stabilizer. In contrast, our research offers a novel perspective by exploring the intrinsic characteristics of unmodified GO. Bulk-scale experiments were conducted using GO particles of different lateral sizes: GO ( ∼ 20 μm), GO-son ( ∼ 500 nm), and NGO ( ∼ 20 nm), at concentrations ranging from 70 ppm to 300 ppm. Our results demonstrate that reducing the particle size of GO significantly improves foam stability by promoting the formation of a network of aggregates at the lamellae and Plateau borders, outperforming the foam produced with larger GO variants. The bulk-scale experiments were further complemented by bubble-scale observations, which revealed that NGO particles pack efficiently at the liquid-air interface, thereby strengthening the lamella structure and preventing Ostwald ripening. Moreover, our results show that the NGO maintains enhanced foam stability even in the presence of decane. Overall, we demonstrate that unmodified GO can effectively stabilize foam at low concentrations, eliminating the need for multi-step chemical modification, which often increases costs and raises environmental concerns.</p><h2>Other Information</h2> <p> Published in: Journal of Molecular Liquids<br> License: <a href="http://creativecommons.org/licenses/by/4.0/" target="_blank">http://creativecommons.org/licenses/by/4.0/</a><br>See article on publisher's website: <a href="https://dx.doi.org/10.1016/j.molliq.2025.128848" target="_blank">https://dx.doi.org/10.1016/j.molliq.2025.128848</a></p>
eu_rights_str_mv openAccess
id Manara2_23c7c6bc1d54b9ce8fa001cf0bc2c7d0
identifier_str_mv 10.1016/j.molliq.2025.128848
network_acronym_str Manara2
network_name_str Manara2
oai_identifier_str oai:figshare.com:article/30636161
publishDate 2025
repository.mail.fl_str_mv
repository.name.fl_str_mv
repository_id_str
rights_invalid_str_mv CC BY 4.0
spelling New insights into the impact of graphene oxide characteristics on foam stability: from bulk behavior to bubble dynamicsAli U. Chaudhry (19724362)Ahmed Abdala (5743205)Rizwan Muneer (19724365)Muhammad Rehan Hashmet (19724368)Thomas Deniel Seers (22631147)Nayef Alyafei (19862553)Reza Sadr (14158884)Harris Sajjad Rabbani (14489205)EngineeringChemical engineeringMaterials engineeringNanotechnologyFoam stabilityNanoparticlesBubble dynamicsNano-graphene oxide<p>Foam stability is critical for various engineering applications. Despite this, foam generated from pure surfactant solutions is often highly unstable, limiting its practical effectiveness. In this study, we investigate the potential of graphene oxide (GO) as an aqueous foam stabilizer under highly saline conditions, using bulk- and bubble-scale experiments. Previous studies have shown that GO, at very low concentrations (∼300 ppm), can negatively impact foam stability, highlighting the importance of surface modification to enhance its performance as a foam stabilizer. In contrast, our research offers a novel perspective by exploring the intrinsic characteristics of unmodified GO. Bulk-scale experiments were conducted using GO particles of different lateral sizes: GO ( ∼ 20 μm), GO-son ( ∼ 500 nm), and NGO ( ∼ 20 nm), at concentrations ranging from 70 ppm to 300 ppm. Our results demonstrate that reducing the particle size of GO significantly improves foam stability by promoting the formation of a network of aggregates at the lamellae and Plateau borders, outperforming the foam produced with larger GO variants. The bulk-scale experiments were further complemented by bubble-scale observations, which revealed that NGO particles pack efficiently at the liquid-air interface, thereby strengthening the lamella structure and preventing Ostwald ripening. Moreover, our results show that the NGO maintains enhanced foam stability even in the presence of decane. Overall, we demonstrate that unmodified GO can effectively stabilize foam at low concentrations, eliminating the need for multi-step chemical modification, which often increases costs and raises environmental concerns.</p><h2>Other Information</h2> <p> Published in: Journal of Molecular Liquids<br> License: <a href="http://creativecommons.org/licenses/by/4.0/" target="_blank">http://creativecommons.org/licenses/by/4.0/</a><br>See article on publisher's website: <a href="https://dx.doi.org/10.1016/j.molliq.2025.128848" target="_blank">https://dx.doi.org/10.1016/j.molliq.2025.128848</a></p>2025-11-10T15:00:00ZTextJournal contributioninfo:eu-repo/semantics/publishedVersiontextcontribution to journal10.1016/j.molliq.2025.128848https://figshare.com/articles/journal_contribution/New_insights_into_the_impact_of_graphene_oxide_characteristics_on_foam_stability_from_bulk_behavior_to_bubble_dynamics/30636161CC BY 4.0info:eu-repo/semantics/openAccessoai:figshare.com:article/306361612025-11-10T15:00:00Z
spellingShingle New insights into the impact of graphene oxide characteristics on foam stability: from bulk behavior to bubble dynamics
Ali U. Chaudhry (19724362)
Engineering
Chemical engineering
Materials engineering
Nanotechnology
Foam stability
Nanoparticles
Bubble dynamics
Nano-graphene oxide
status_str publishedVersion
title New insights into the impact of graphene oxide characteristics on foam stability: from bulk behavior to bubble dynamics
title_full New insights into the impact of graphene oxide characteristics on foam stability: from bulk behavior to bubble dynamics
title_fullStr New insights into the impact of graphene oxide characteristics on foam stability: from bulk behavior to bubble dynamics
title_full_unstemmed New insights into the impact of graphene oxide characteristics on foam stability: from bulk behavior to bubble dynamics
title_short New insights into the impact of graphene oxide characteristics on foam stability: from bulk behavior to bubble dynamics
title_sort New insights into the impact of graphene oxide characteristics on foam stability: from bulk behavior to bubble dynamics
topic Engineering
Chemical engineering
Materials engineering
Nanotechnology
Foam stability
Nanoparticles
Bubble dynamics
Nano-graphene oxide