Permeabilities of CO<sub>2</sub>, H<sub>2</sub>S and CH<sub>4</sub> through Choline-Based Ionic Liquids: Atomistic-Scale Simulations

<p dir="ltr">Molecular dynamics simulations are used to study the transport of CO<sub>2</sub> , H<sub>2</sub>S and CH<sub>4</sub> molecules across environmentally friendly choline-benzoate and choline-lactate ionic liquids (ILs). The permeability c...

وصف كامل

محفوظ في:
التفاصيل البيبلوغرافية
المؤلف الرئيسي: Abdukarem Amhamed (14603357) (author)
مؤلفون آخرون: Mert Atilhan (1272906) (author), Golibjon Berdiyorov (6325997) (author)
منشور في: 2019
الموضوعات:
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author Abdukarem Amhamed (14603357)
author2 Mert Atilhan (1272906)
Golibjon Berdiyorov (6325997)
author2_role author
author
author_facet Abdukarem Amhamed (14603357)
Mert Atilhan (1272906)
Golibjon Berdiyorov (6325997)
author_role author
dc.creator.none.fl_str_mv Abdukarem Amhamed (14603357)
Mert Atilhan (1272906)
Golibjon Berdiyorov (6325997)
dc.date.none.fl_str_mv 2019-05-27T03:00:00Z
dc.identifier.none.fl_str_mv 10.3390/molecules24102014
dc.relation.none.fl_str_mv https://figshare.com/articles/journal_contribution/Permeabilities_of_CO_sub_2_sub_H_sub_2_sub_S_and_CH_sub_4_sub_through_Choline-Based_Ionic_Liquids_Atomistic-Scale_Simulations/25348261
dc.rights.none.fl_str_mv CC BY 4.0
info:eu-repo/semantics/openAccess
dc.subject.none.fl_str_mv Biomedical and clinical sciences
Pharmacology and pharmaceutical sciences
Chemical sciences
Analytical chemistry
Organic chemistry
Theoretical and computational chemistry
ionic liquid
gas separation
molecular dynamics
dc.title.none.fl_str_mv Permeabilities of CO<sub>2</sub>, H<sub>2</sub>S and CH<sub>4</sub> through Choline-Based Ionic Liquids: Atomistic-Scale Simulations
dc.type.none.fl_str_mv Text
Journal contribution
info:eu-repo/semantics/publishedVersion
text
contribution to journal
description <p dir="ltr">Molecular dynamics simulations are used to study the transport of CO<sub>2</sub> , H<sub>2</sub>S and CH<sub>4</sub> molecules across environmentally friendly choline-benzoate and choline-lactate ionic liquids (ILs). The permeability coefficients of the considered molecules are calculated using the free energy and diffusion rate profiles. Both systems show the largest resistance to CH<sub>4</sub> , whereas more than 5 orders of magnitude larger permeability coefficients are obtained for the other two gas molecules. The CO<sub>2</sub> /CH<sub>4</sub> and H<sub>2</sub>S/CH<sub>4</sub> selectivity was estimated to be more than 10<sup>4</sup> and 10<sup>5</sup> , respectively. These results indicate the great potential of the considered ILs for greenhouse gas control.</p><p><br></p><h2>Other Information</h2><p dir="ltr">Published in: Molecules<br>License: <a href="https://creativecommons.org/licenses/by/4.0/" target="_blank">https://creativecommons.org/licenses/by/4.0/</a><br>See article on publisher's website: <a href="https://dx.doi.org/10.3390/molecules24102014" target="_blank">https://dx.doi.org/10.3390/molecules24102014</a></p>
eu_rights_str_mv openAccess
id Manara2_2853c0764859b49402ada579ecaeb5be
identifier_str_mv 10.3390/molecules24102014
network_acronym_str Manara2
network_name_str Manara2
oai_identifier_str oai:figshare.com:article/25348261
publishDate 2019
repository.mail.fl_str_mv
repository.name.fl_str_mv
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rights_invalid_str_mv CC BY 4.0
spelling Permeabilities of CO<sub>2</sub>, H<sub>2</sub>S and CH<sub>4</sub> through Choline-Based Ionic Liquids: Atomistic-Scale SimulationsAbdukarem Amhamed (14603357)Mert Atilhan (1272906)Golibjon Berdiyorov (6325997)Biomedical and clinical sciencesPharmacology and pharmaceutical sciencesChemical sciencesAnalytical chemistryOrganic chemistryTheoretical and computational chemistryionic liquidgas separationmolecular dynamics<p dir="ltr">Molecular dynamics simulations are used to study the transport of CO<sub>2</sub> , H<sub>2</sub>S and CH<sub>4</sub> molecules across environmentally friendly choline-benzoate and choline-lactate ionic liquids (ILs). The permeability coefficients of the considered molecules are calculated using the free energy and diffusion rate profiles. Both systems show the largest resistance to CH<sub>4</sub> , whereas more than 5 orders of magnitude larger permeability coefficients are obtained for the other two gas molecules. The CO<sub>2</sub> /CH<sub>4</sub> and H<sub>2</sub>S/CH<sub>4</sub> selectivity was estimated to be more than 10<sup>4</sup> and 10<sup>5</sup> , respectively. These results indicate the great potential of the considered ILs for greenhouse gas control.</p><p><br></p><h2>Other Information</h2><p dir="ltr">Published in: Molecules<br>License: <a href="https://creativecommons.org/licenses/by/4.0/" target="_blank">https://creativecommons.org/licenses/by/4.0/</a><br>See article on publisher's website: <a href="https://dx.doi.org/10.3390/molecules24102014" target="_blank">https://dx.doi.org/10.3390/molecules24102014</a></p>2019-05-27T03:00:00ZTextJournal contributioninfo:eu-repo/semantics/publishedVersiontextcontribution to journal10.3390/molecules24102014https://figshare.com/articles/journal_contribution/Permeabilities_of_CO_sub_2_sub_H_sub_2_sub_S_and_CH_sub_4_sub_through_Choline-Based_Ionic_Liquids_Atomistic-Scale_Simulations/25348261CC BY 4.0info:eu-repo/semantics/openAccessoai:figshare.com:article/253482612019-05-27T03:00:00Z
spellingShingle Permeabilities of CO<sub>2</sub>, H<sub>2</sub>S and CH<sub>4</sub> through Choline-Based Ionic Liquids: Atomistic-Scale Simulations
Abdukarem Amhamed (14603357)
Biomedical and clinical sciences
Pharmacology and pharmaceutical sciences
Chemical sciences
Analytical chemistry
Organic chemistry
Theoretical and computational chemistry
ionic liquid
gas separation
molecular dynamics
status_str publishedVersion
title Permeabilities of CO<sub>2</sub>, H<sub>2</sub>S and CH<sub>4</sub> through Choline-Based Ionic Liquids: Atomistic-Scale Simulations
title_full Permeabilities of CO<sub>2</sub>, H<sub>2</sub>S and CH<sub>4</sub> through Choline-Based Ionic Liquids: Atomistic-Scale Simulations
title_fullStr Permeabilities of CO<sub>2</sub>, H<sub>2</sub>S and CH<sub>4</sub> through Choline-Based Ionic Liquids: Atomistic-Scale Simulations
title_full_unstemmed Permeabilities of CO<sub>2</sub>, H<sub>2</sub>S and CH<sub>4</sub> through Choline-Based Ionic Liquids: Atomistic-Scale Simulations
title_short Permeabilities of CO<sub>2</sub>, H<sub>2</sub>S and CH<sub>4</sub> through Choline-Based Ionic Liquids: Atomistic-Scale Simulations
title_sort Permeabilities of CO<sub>2</sub>, H<sub>2</sub>S and CH<sub>4</sub> through Choline-Based Ionic Liquids: Atomistic-Scale Simulations
topic Biomedical and clinical sciences
Pharmacology and pharmaceutical sciences
Chemical sciences
Analytical chemistry
Organic chemistry
Theoretical and computational chemistry
ionic liquid
gas separation
molecular dynamics