Development of eco-friendly coating for the fabrication of high performing loose nanofiltration membranes for dye-contaminated wastewater treatment

<p>This study introduces highly efficient loose nanofiltration (LNF) membranes developed through a green synergistic combination of tannic acid (TA) and polyvinyl alcohol (PVA), aimed at addressing the complex challenge of dye/salt fractionation in wastewater treatment. Utilizing a one-step co...

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محفوظ في:
التفاصيل البيبلوغرافية
المؤلف الرئيسي: Abedalkader Alkhouzaam (15842647) (author)
مؤلفون آخرون: Marwan Khraisheh (15842653) (author)
منشور في: 2024
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author Abedalkader Alkhouzaam (15842647)
author2 Marwan Khraisheh (15842653)
author2_role author
author_facet Abedalkader Alkhouzaam (15842647)
Marwan Khraisheh (15842653)
author_role author
dc.creator.none.fl_str_mv Abedalkader Alkhouzaam (15842647)
Marwan Khraisheh (15842653)
dc.date.none.fl_str_mv 2024-07-20T03:00:00Z
dc.identifier.none.fl_str_mv 10.1016/j.desal.2024.117609
dc.relation.none.fl_str_mv https://figshare.com/articles/journal_contribution/Development_of_eco-friendly_coating_for_the_fabrication_of_high_performing_loose_nanofiltration_membranes_for_dye-contaminated_wastewater_treatment/25827085
dc.rights.none.fl_str_mv CC BY 4.0
info:eu-repo/semantics/openAccess
dc.subject.none.fl_str_mv Engineering
Chemical engineering
Environmental engineering
Loose nanofiltration
Dye/salt separation
Low pressure
Tannic acid
Antifouling membrane
dc.title.none.fl_str_mv Development of eco-friendly coating for the fabrication of high performing loose nanofiltration membranes for dye-contaminated wastewater treatment
dc.type.none.fl_str_mv Text
Journal contribution
info:eu-repo/semantics/publishedVersion
text
contribution to journal
description <p>This study introduces highly efficient loose nanofiltration (LNF) membranes developed through a green synergistic combination of tannic acid (TA) and polyvinyl alcohol (PVA), aimed at addressing the complex challenge of dye/salt fractionation in wastewater treatment. Utilizing a one-step co-deposition technique onto a polysulfone (PSF) substrate, the integration of TA and PVA has produced membranes with excellent functional capabilities. Comprehensive chemical analyses, including FTIR and XPS, confirm the successful integration and chemical modification of TA, leading to enhanced membrane functionality. This is further evidenced by SEM, MWCO, and contact angle measurements, which reveal decreased pore size and increased hydrophilicity. The TA/PVA-coated membranes demonstrated high water permeability up to 138 LMH/bar and excellent dye/salt selectivity, achieving ~99 % Congo Red (CR) rejection with <10 % salt rejection in both single-component and dye/salt mixture filtrations. Notably, these membranes exhibited remarkable fouling resistance, with Flux Recovery Ratios (FRR) up to 99 % against dye/salt mixtures. This eco-friendly approach, leveraging the green chemistry of TA and PVA, offers a cost-effective solution to one of the most challenging wastewaters in membrane technology.</p><h2>Other Information</h2> <p> Published in: Desalination<br> License: <a href="http://creativecommons.org/licenses/by/4.0/" target="_blank">http://creativecommons.org/licenses/by/4.0/</a><br>See article on publisher's website: <a href="https://dx.doi.org/10.1016/j.desal.2024.117609" target="_blank">https://dx.doi.org/10.1016/j.desal.2024.117609</a></p>
eu_rights_str_mv openAccess
id Manara2_3f3405976c3604eabeeb3e509975dcb5
identifier_str_mv 10.1016/j.desal.2024.117609
network_acronym_str Manara2
network_name_str Manara2
oai_identifier_str oai:figshare.com:article/25827085
publishDate 2024
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spelling Development of eco-friendly coating for the fabrication of high performing loose nanofiltration membranes for dye-contaminated wastewater treatmentAbedalkader Alkhouzaam (15842647)Marwan Khraisheh (15842653)EngineeringChemical engineeringEnvironmental engineeringLoose nanofiltrationDye/salt separationLow pressureTannic acidAntifouling membrane<p>This study introduces highly efficient loose nanofiltration (LNF) membranes developed through a green synergistic combination of tannic acid (TA) and polyvinyl alcohol (PVA), aimed at addressing the complex challenge of dye/salt fractionation in wastewater treatment. Utilizing a one-step co-deposition technique onto a polysulfone (PSF) substrate, the integration of TA and PVA has produced membranes with excellent functional capabilities. Comprehensive chemical analyses, including FTIR and XPS, confirm the successful integration and chemical modification of TA, leading to enhanced membrane functionality. This is further evidenced by SEM, MWCO, and contact angle measurements, which reveal decreased pore size and increased hydrophilicity. The TA/PVA-coated membranes demonstrated high water permeability up to 138 LMH/bar and excellent dye/salt selectivity, achieving ~99 % Congo Red (CR) rejection with <10 % salt rejection in both single-component and dye/salt mixture filtrations. Notably, these membranes exhibited remarkable fouling resistance, with Flux Recovery Ratios (FRR) up to 99 % against dye/salt mixtures. This eco-friendly approach, leveraging the green chemistry of TA and PVA, offers a cost-effective solution to one of the most challenging wastewaters in membrane technology.</p><h2>Other Information</h2> <p> Published in: Desalination<br> License: <a href="http://creativecommons.org/licenses/by/4.0/" target="_blank">http://creativecommons.org/licenses/by/4.0/</a><br>See article on publisher's website: <a href="https://dx.doi.org/10.1016/j.desal.2024.117609" target="_blank">https://dx.doi.org/10.1016/j.desal.2024.117609</a></p>2024-07-20T03:00:00ZTextJournal contributioninfo:eu-repo/semantics/publishedVersiontextcontribution to journal10.1016/j.desal.2024.117609https://figshare.com/articles/journal_contribution/Development_of_eco-friendly_coating_for_the_fabrication_of_high_performing_loose_nanofiltration_membranes_for_dye-contaminated_wastewater_treatment/25827085CC BY 4.0info:eu-repo/semantics/openAccessoai:figshare.com:article/258270852024-07-20T03:00:00Z
spellingShingle Development of eco-friendly coating for the fabrication of high performing loose nanofiltration membranes for dye-contaminated wastewater treatment
Abedalkader Alkhouzaam (15842647)
Engineering
Chemical engineering
Environmental engineering
Loose nanofiltration
Dye/salt separation
Low pressure
Tannic acid
Antifouling membrane
status_str publishedVersion
title Development of eco-friendly coating for the fabrication of high performing loose nanofiltration membranes for dye-contaminated wastewater treatment
title_full Development of eco-friendly coating for the fabrication of high performing loose nanofiltration membranes for dye-contaminated wastewater treatment
title_fullStr Development of eco-friendly coating for the fabrication of high performing loose nanofiltration membranes for dye-contaminated wastewater treatment
title_full_unstemmed Development of eco-friendly coating for the fabrication of high performing loose nanofiltration membranes for dye-contaminated wastewater treatment
title_short Development of eco-friendly coating for the fabrication of high performing loose nanofiltration membranes for dye-contaminated wastewater treatment
title_sort Development of eco-friendly coating for the fabrication of high performing loose nanofiltration membranes for dye-contaminated wastewater treatment
topic Engineering
Chemical engineering
Environmental engineering
Loose nanofiltration
Dye/salt separation
Low pressure
Tannic acid
Antifouling membrane