Optical properties of functionalized Ti<sub>3</sub>C<sub>2</sub>T<sub>2</sub> (T = F, O, OH) MXene: First-principles calculations

<p dir="ltr">Role of surface termination on the dielectric and optical properties of Ti3C2T2 (T = F, O, OH) MXene is studied using first-principles density functional theory. The results show that the surface functionalization has a significant impact on the optical properties of the...

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المؤلف الرئيسي: G. R. Berdiyorov (4435975) (author)
منشور في: 2016
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author G. R. Berdiyorov (4435975)
author_facet G. R. Berdiyorov (4435975)
author_role author
dc.creator.none.fl_str_mv G. R. Berdiyorov (4435975)
dc.date.none.fl_str_mv 2016-05-03T03:00:00Z
dc.identifier.none.fl_str_mv 10.1063/1.4948799
dc.relation.none.fl_str_mv https://figshare.com/articles/journal_contribution/Optical_properties_of_functionalized_Ti3C2T2_T_F_O_OH_MXene_First-principles_calculations/27094510
dc.rights.none.fl_str_mv CC BY 4.0
info:eu-repo/semantics/openAccess
dc.subject.none.fl_str_mv Chemical sciences
Theoretical and computational chemistry
Engineering
Materials engineering
Nanotechnology
Dielectric properties
Optical properties
MXenes
Surface termination
Density functional theory
dc.title.none.fl_str_mv Optical properties of functionalized Ti<sub>3</sub>C<sub>2</sub>T<sub>2</sub> (T = F, O, OH) MXene: First-principles calculations
dc.type.none.fl_str_mv Text
Journal contribution
info:eu-repo/semantics/publishedVersion
text
contribution to journal
description <p dir="ltr">Role of surface termination on the dielectric and optical properties of Ti3C2T2 (T = F, O, OH) MXene is studied using first-principles density functional theory. The results show that the surface functionalization has a significant impact on the optical properties of the MXene. For example, in the visible range of the spectrum, the oxidized sample shows larger absorption, whereas surface fluorination results in weaker absorption as compared to pristine MXene. In the ultraviolet energy range, all functional groups lead to the enhancement of both absorption and reflectivity of the material. Dielectric properties of MXene are also sensitive to the surface functionalization. Our findings demonstrate the importance of surface termination on the optical properties of the MXene.</p><h2>Other Information</h2><p dir="ltr">Published in: AIP Advances<br>License: <a href="https://creativecommons.org/licenses/by/4.0/deed.en" rel="noreferrer noopener" target="_blank">https://creativecommons.org/licenses/by/4.0/</a>  <br>See article on publisher's website: <a href="https://dx.doi.org/10.1063/1.4948799" target="_blank">https://dx.doi.org/10.1063/1.4948799</a></p>
eu_rights_str_mv openAccess
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identifier_str_mv 10.1063/1.4948799
network_acronym_str Manara2
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oai_identifier_str oai:figshare.com:article/27094510
publishDate 2016
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spelling Optical properties of functionalized Ti<sub>3</sub>C<sub>2</sub>T<sub>2</sub> (T = F, O, OH) MXene: First-principles calculationsG. R. Berdiyorov (4435975)Chemical sciencesTheoretical and computational chemistryEngineeringMaterials engineeringNanotechnologyDielectric propertiesOptical propertiesMXenesSurface terminationDensity functional theory<p dir="ltr">Role of surface termination on the dielectric and optical properties of Ti3C2T2 (T = F, O, OH) MXene is studied using first-principles density functional theory. The results show that the surface functionalization has a significant impact on the optical properties of the MXene. For example, in the visible range of the spectrum, the oxidized sample shows larger absorption, whereas surface fluorination results in weaker absorption as compared to pristine MXene. In the ultraviolet energy range, all functional groups lead to the enhancement of both absorption and reflectivity of the material. Dielectric properties of MXene are also sensitive to the surface functionalization. Our findings demonstrate the importance of surface termination on the optical properties of the MXene.</p><h2>Other Information</h2><p dir="ltr">Published in: AIP Advances<br>License: <a href="https://creativecommons.org/licenses/by/4.0/deed.en" rel="noreferrer noopener" target="_blank">https://creativecommons.org/licenses/by/4.0/</a>  <br>See article on publisher's website: <a href="https://dx.doi.org/10.1063/1.4948799" target="_blank">https://dx.doi.org/10.1063/1.4948799</a></p>2016-05-03T03:00:00ZTextJournal contributioninfo:eu-repo/semantics/publishedVersiontextcontribution to journal10.1063/1.4948799https://figshare.com/articles/journal_contribution/Optical_properties_of_functionalized_Ti3C2T2_T_F_O_OH_MXene_First-principles_calculations/27094510CC BY 4.0info:eu-repo/semantics/openAccessoai:figshare.com:article/270945102016-05-03T03:00:00Z
spellingShingle Optical properties of functionalized Ti<sub>3</sub>C<sub>2</sub>T<sub>2</sub> (T = F, O, OH) MXene: First-principles calculations
G. R. Berdiyorov (4435975)
Chemical sciences
Theoretical and computational chemistry
Engineering
Materials engineering
Nanotechnology
Dielectric properties
Optical properties
MXenes
Surface termination
Density functional theory
status_str publishedVersion
title Optical properties of functionalized Ti<sub>3</sub>C<sub>2</sub>T<sub>2</sub> (T = F, O, OH) MXene: First-principles calculations
title_full Optical properties of functionalized Ti<sub>3</sub>C<sub>2</sub>T<sub>2</sub> (T = F, O, OH) MXene: First-principles calculations
title_fullStr Optical properties of functionalized Ti<sub>3</sub>C<sub>2</sub>T<sub>2</sub> (T = F, O, OH) MXene: First-principles calculations
title_full_unstemmed Optical properties of functionalized Ti<sub>3</sub>C<sub>2</sub>T<sub>2</sub> (T = F, O, OH) MXene: First-principles calculations
title_short Optical properties of functionalized Ti<sub>3</sub>C<sub>2</sub>T<sub>2</sub> (T = F, O, OH) MXene: First-principles calculations
title_sort Optical properties of functionalized Ti<sub>3</sub>C<sub>2</sub>T<sub>2</sub> (T = F, O, OH) MXene: First-principles calculations
topic Chemical sciences
Theoretical and computational chemistry
Engineering
Materials engineering
Nanotechnology
Dielectric properties
Optical properties
MXenes
Surface termination
Density functional theory