Evaluation of method performance and matrix effect for 57 commonly used herbicides in some vegetable families using LC-MS/MS determination

<p dir="ltr">A modified QuEChERS method was employed with LC-MS/MS to evaluate the matrix effects of 12 different vegetables matrices in 57 globally used herbicides. The average recoveries of pesticides at different concentrations varied between 70 and 120%. The reproducibility expre...

وصف كامل

محفوظ في:
التفاصيل البيبلوغرافية
المؤلف الرئيسي: Ali S. Mohammed (9352461) (author)
مؤلفون آخرون: Gouda A. Ramadan (9352464) (author), Ahmed I. Abdelkader (9352467) (author), Sohair A. Gadalla (9352470) (author), Mohsen M. Ayoub (9352473) (author), Najat A. Alabdulmalik (9352476) (author), Wasan A. AL Baker (20362830) (author)
منشور في: 2020
الموضوعات:
الوسوم: إضافة وسم
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الوصف
الملخص:<p dir="ltr">A modified QuEChERS method was employed with LC-MS/MS to evaluate the matrix effects of 12 different vegetables matrices in 57 globally used herbicides. The average recoveries of pesticides at different concentrations varied between 70 and 120%. The reproducibility expressed as relative standard deviation was <25%. The limit of quantitation was (0.005–0.01 mg/kg). The measurement uncertainty is lower than 40%. Three vegetables families: Cucurbitaceae, Solanaceae and leafy vegetables were selectd for study. Among the investigated commodities, leafy green vegetables have the highest matrix effects, MEs percentages ranged between (2 & 282%). The highest suppression in analytes response was observed for parsley with matrix ME (2–19%). Most of tested herbicides showed suppression extent at the lower fortified concentrations. Tomato recorded the highest enhancement in most of studied herbicides of MEs% ranged from (122 to 379%). Butachlor, chlorbromuron, fenoxaprop-p-ethyl, flufenacet, fluzafop-p-butyl, hexythiazox, prosulfocarb and pyriproxyfen showed ion suppresion for all vegetables matrices with MEs% ranged from (5 to 79%). Matrix effects (MEs) were evaluated by comparing the slopes of target analytes to prove reproducibility (n = 5). The current study emphasize using of matrix match calibration with these commodity pesticides combinations, whereas, ME’s were dependent on composition of analyte and co-eluting agents.</p><h2>Other Information</h2><p dir="ltr">Published in: Cogent Food & Agriculture<br>License: <a href="http://creativecommons.org/licenses/by/4.0/" target="_blank">http://creativecommons.org/licenses/by/4.0/</a><br>See article on publisher's website: <a href="https://dx.doi.org/10.1080/23311932.2020.1815287" target="_blank">https://dx.doi.org/10.1080/23311932.2020.1815287</a></p>