Dynamic 3D imaging of gas hydrate kinetics using synchrotron computed tomography

<p dir="ltr">The availability of natural gas hydrates and the continuing increase in energy demand, motivated researchers to consider gas hydrates as a future source of energy. Fundamental understanding of hydrate dissociation kinetics is essential to improve techniques of gas produc...

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Main Author: Zaher Jarrar (18805912) (author)
Other Authors: Riyadh Al-Raoush (18805915) (author), Khalid Alshibli (18805918) (author), Jongwon Jung (9641431) (author)
Published: 2020
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author Zaher Jarrar (18805912)
author2 Riyadh Al-Raoush (18805915)
Khalid Alshibli (18805918)
Jongwon Jung (9641431)
author2_role author
author
author
author_facet Zaher Jarrar (18805912)
Riyadh Al-Raoush (18805915)
Khalid Alshibli (18805918)
Jongwon Jung (9641431)
author_role author
dc.creator.none.fl_str_mv Zaher Jarrar (18805912)
Riyadh Al-Raoush (18805915)
Khalid Alshibli (18805918)
Jongwon Jung (9641431)
dc.date.none.fl_str_mv 2020-11-01T00:00:00Z
dc.identifier.none.fl_str_mv 10.1051/e3sconf/202020511004
dc.relation.none.fl_str_mv https://figshare.com/articles/journal_contribution/Dynamic_3D_imaging_of_gas_hydrate_kinetics_using_synchrotron_computed_tomography/26015815
dc.rights.none.fl_str_mv CC BY 4.0
info:eu-repo/semantics/openAccess
dc.subject.none.fl_str_mv Engineering
Geomatic engineering
Resources engineering and extractive metallurgy
Gas hydrates
Energy resources
Xenon hydrate
Hydrate formation
Surface area evolution
Natural hydrate reservoirs
Energy production techniques
dc.title.none.fl_str_mv Dynamic 3D imaging of gas hydrate kinetics using synchrotron computed tomography
dc.type.none.fl_str_mv Text
Journal contribution
info:eu-repo/semantics/publishedVersion
text
contribution to journal
description <p dir="ltr">The availability of natural gas hydrates and the continuing increase in energy demand, motivated researchers to consider gas hydrates as a future source of energy. Fundamental understanding of hydrate dissociation kinetics is essential to improve techniques of gas production from natural hydrates reservoirs. During hydrate dissociation, bonds between water (host molecules) and gas (guest molecules) break and free gas is released. This paper investigates the evolution of hydrate surface area, pore habit, and tortuosity using in-situ imaging of Xenon (Xe) hydrate formation and dissociation in porous media with dynamic three-dimensional synchrotron microcomputed tomography (SMT). Xe hydrate was formed inside a high- pressure, low-temperature cell and then dissociated by thermal stimulation. During formation and dissociation, full 3D SMT scans were acquired continuously and reconstructed into 3D volume images. Each scan took only 45 seconds to complete, and a total of 60 scans were acquired. Hydrate volume and surface area evolution were directly measured from the SMT scans. At low hydrate saturation, the predominant pore habit was surface coating, while the predominant pore habit at high hydrate saturation was pore filling. A second-degree polynomial can be used to predict variation of tortuosity with hydrate saturation with an R2 value of 0.997.</p><h2>Other Information</h2><p dir="ltr">Published in: E3S Web of Conferences<br>License: <a href="https://creativecommons.org/licenses/by/4.0/" target="_blank">https://creativecommons.org/licenses/by/4.0/</a><br>See article on publisher's website: <a href="https://dx.doi.org/10.1051/e3sconf/202020511004" target="_blank">https://dx.doi.org/10.1051/e3sconf/202020511004</a></p>
eu_rights_str_mv openAccess
id Manara2_91324692e5d9a59ef207d13a3f5fb925
identifier_str_mv 10.1051/e3sconf/202020511004
network_acronym_str Manara2
network_name_str Manara2
oai_identifier_str oai:figshare.com:article/26015815
publishDate 2020
repository.mail.fl_str_mv
repository.name.fl_str_mv
repository_id_str
rights_invalid_str_mv CC BY 4.0
spelling Dynamic 3D imaging of gas hydrate kinetics using synchrotron computed tomographyZaher Jarrar (18805912)Riyadh Al-Raoush (18805915)Khalid Alshibli (18805918)Jongwon Jung (9641431)EngineeringGeomatic engineeringResources engineering and extractive metallurgyGas hydratesEnergy resourcesXenon hydrateHydrate formationSurface area evolutionNatural hydrate reservoirsEnergy production techniques<p dir="ltr">The availability of natural gas hydrates and the continuing increase in energy demand, motivated researchers to consider gas hydrates as a future source of energy. Fundamental understanding of hydrate dissociation kinetics is essential to improve techniques of gas production from natural hydrates reservoirs. During hydrate dissociation, bonds between water (host molecules) and gas (guest molecules) break and free gas is released. This paper investigates the evolution of hydrate surface area, pore habit, and tortuosity using in-situ imaging of Xenon (Xe) hydrate formation and dissociation in porous media with dynamic three-dimensional synchrotron microcomputed tomography (SMT). Xe hydrate was formed inside a high- pressure, low-temperature cell and then dissociated by thermal stimulation. During formation and dissociation, full 3D SMT scans were acquired continuously and reconstructed into 3D volume images. Each scan took only 45 seconds to complete, and a total of 60 scans were acquired. Hydrate volume and surface area evolution were directly measured from the SMT scans. At low hydrate saturation, the predominant pore habit was surface coating, while the predominant pore habit at high hydrate saturation was pore filling. A second-degree polynomial can be used to predict variation of tortuosity with hydrate saturation with an R2 value of 0.997.</p><h2>Other Information</h2><p dir="ltr">Published in: E3S Web of Conferences<br>License: <a href="https://creativecommons.org/licenses/by/4.0/" target="_blank">https://creativecommons.org/licenses/by/4.0/</a><br>See article on publisher's website: <a href="https://dx.doi.org/10.1051/e3sconf/202020511004" target="_blank">https://dx.doi.org/10.1051/e3sconf/202020511004</a></p>2020-11-01T00:00:00ZTextJournal contributioninfo:eu-repo/semantics/publishedVersiontextcontribution to journal10.1051/e3sconf/202020511004https://figshare.com/articles/journal_contribution/Dynamic_3D_imaging_of_gas_hydrate_kinetics_using_synchrotron_computed_tomography/26015815CC BY 4.0info:eu-repo/semantics/openAccessoai:figshare.com:article/260158152020-11-01T00:00:00Z
spellingShingle Dynamic 3D imaging of gas hydrate kinetics using synchrotron computed tomography
Zaher Jarrar (18805912)
Engineering
Geomatic engineering
Resources engineering and extractive metallurgy
Gas hydrates
Energy resources
Xenon hydrate
Hydrate formation
Surface area evolution
Natural hydrate reservoirs
Energy production techniques
status_str publishedVersion
title Dynamic 3D imaging of gas hydrate kinetics using synchrotron computed tomography
title_full Dynamic 3D imaging of gas hydrate kinetics using synchrotron computed tomography
title_fullStr Dynamic 3D imaging of gas hydrate kinetics using synchrotron computed tomography
title_full_unstemmed Dynamic 3D imaging of gas hydrate kinetics using synchrotron computed tomography
title_short Dynamic 3D imaging of gas hydrate kinetics using synchrotron computed tomography
title_sort Dynamic 3D imaging of gas hydrate kinetics using synchrotron computed tomography
topic Engineering
Geomatic engineering
Resources engineering and extractive metallurgy
Gas hydrates
Energy resources
Xenon hydrate
Hydrate formation
Surface area evolution
Natural hydrate reservoirs
Energy production techniques