Influence of polymer structure and amount on microstructure and properties of polyethylene-modified asphalt binders

<p>In recent years, the use of polyethylene (PE) for asphalt modification has been gaining increased attention due to the environmental sustainability and cost-saving benefits. To optimize the performance of the PE-asphalt blends, it is necessary to understand the polymer-binder interactions a...

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التفاصيل البيبلوغرافية
المؤلف الرئيسي: K. Lakshmi Roja (14159028) (author)
مؤلفون آخرون: Amara Rehman (14153475) (author), Mabrouk Ouederni (14153478) (author), Senthil Kumar Krishnamoorthy (14153481) (author), Ahmed Abdala (5743205) (author), Eyad Masad (14153484) (author)
منشور في: 2022
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author K. Lakshmi Roja (14159028)
author2 Amara Rehman (14153475)
Mabrouk Ouederni (14153478)
Senthil Kumar Krishnamoorthy (14153481)
Ahmed Abdala (5743205)
Eyad Masad (14153484)
author2_role author
author
author
author
author
author_facet K. Lakshmi Roja (14159028)
Amara Rehman (14153475)
Mabrouk Ouederni (14153478)
Senthil Kumar Krishnamoorthy (14153481)
Ahmed Abdala (5743205)
Eyad Masad (14153484)
author_role author
dc.creator.none.fl_str_mv K. Lakshmi Roja (14159028)
Amara Rehman (14153475)
Mabrouk Ouederni (14153478)
Senthil Kumar Krishnamoorthy (14153481)
Ahmed Abdala (5743205)
Eyad Masad (14153484)
dc.date.none.fl_str_mv 2022-11-22T21:18:36Z
dc.identifier.none.fl_str_mv 10.1617/s11527-021-01683-0
dc.relation.none.fl_str_mv https://figshare.com/articles/journal_contribution/Influence_of_polymer_structure_and_amount_on_microstructure_and_properties_of_polyethylene-modified_asphalt_binders/21598560
dc.rights.none.fl_str_mv CC BY 4.0
info:eu-repo/semantics/openAccess
dc.subject.none.fl_str_mv Macromolecular and materials chemistry
Materials engineering
Mechanics of Materials
General Materials Science
Building and Construction
Civil and Structural Engineering
dc.title.none.fl_str_mv Influence of polymer structure and amount on microstructure and properties of polyethylene-modified asphalt binders
dc.type.none.fl_str_mv Text
Journal contribution
info:eu-repo/semantics/publishedVersion
text
contribution to journal
description <p>In recent years, the use of polyethylene (PE) for asphalt modification has been gaining increased attention due to the environmental sustainability and cost-saving benefits. To optimize the performance of the PE-asphalt blends, it is necessary to understand the polymer-binder interactions and their impact on the properties of the modified asphalt binder. In this study, low-density polyethylene (LDPE) with low and high melt flow index (MFI), i.e., LDPE4 and LDPE70, were blended with Pen 60-70 asphalt binder in dosages ranging from 1 to 5 wt.%. PE Wax was also added to the binder or the PE-binder blend to enhance dispersion. The dispersion of PE in the binder and the phase stability of the modified binder were investigated by optical microscope. The equivalent diameter of PE domains increased with time and the polymer dosage level. The addition of PE wax improved the polymer dispersity in the LDPE4 blends. The polymer dispersity in LDPE70 blends was good without adding PE Wax, attributed to the higher MFI value (low molecular weight) of LDPE70. In addition, to understand the stability of polymer modified binder, the steady shear viscosity-temperature profile of these binders was studied using a rotational viscometer. The dynamic rheological properties and performance of the PE-binder blends were evaluated using the dynamic shear rheometer. Based on the microstructure, all other rheological and performance properties, it was concluded that the 3% LDPE70 binder has better polymer dispersity, better low and high temperature performance characteristics.</p><h2>Other Information</h2> <p> Published in: Materials and Structures<br> License: <a href="https://creativecommons.org/licenses/by/4.0" target="_blank">https://creativecommons.org/licenses/by/4.0</a><br>See article on publisher's website: <a href="http://dx.doi.org/10.1617/s11527-021-01683-0" target="_blank">http://dx.doi.org/10.1617/s11527-021-01683-0</a></p>
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identifier_str_mv 10.1617/s11527-021-01683-0
network_acronym_str Manara2
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oai_identifier_str oai:figshare.com:article/21598560
publishDate 2022
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spelling Influence of polymer structure and amount on microstructure and properties of polyethylene-modified asphalt bindersK. Lakshmi Roja (14159028)Amara Rehman (14153475)Mabrouk Ouederni (14153478)Senthil Kumar Krishnamoorthy (14153481)Ahmed Abdala (5743205)Eyad Masad (14153484)Macromolecular and materials chemistryMaterials engineeringMechanics of MaterialsGeneral Materials ScienceBuilding and ConstructionCivil and Structural Engineering<p>In recent years, the use of polyethylene (PE) for asphalt modification has been gaining increased attention due to the environmental sustainability and cost-saving benefits. To optimize the performance of the PE-asphalt blends, it is necessary to understand the polymer-binder interactions and their impact on the properties of the modified asphalt binder. In this study, low-density polyethylene (LDPE) with low and high melt flow index (MFI), i.e., LDPE4 and LDPE70, were blended with Pen 60-70 asphalt binder in dosages ranging from 1 to 5 wt.%. PE Wax was also added to the binder or the PE-binder blend to enhance dispersion. The dispersion of PE in the binder and the phase stability of the modified binder were investigated by optical microscope. The equivalent diameter of PE domains increased with time and the polymer dosage level. The addition of PE wax improved the polymer dispersity in the LDPE4 blends. The polymer dispersity in LDPE70 blends was good without adding PE Wax, attributed to the higher MFI value (low molecular weight) of LDPE70. In addition, to understand the stability of polymer modified binder, the steady shear viscosity-temperature profile of these binders was studied using a rotational viscometer. The dynamic rheological properties and performance of the PE-binder blends were evaluated using the dynamic shear rheometer. Based on the microstructure, all other rheological and performance properties, it was concluded that the 3% LDPE70 binder has better polymer dispersity, better low and high temperature performance characteristics.</p><h2>Other Information</h2> <p> Published in: Materials and Structures<br> License: <a href="https://creativecommons.org/licenses/by/4.0" target="_blank">https://creativecommons.org/licenses/by/4.0</a><br>See article on publisher's website: <a href="http://dx.doi.org/10.1617/s11527-021-01683-0" target="_blank">http://dx.doi.org/10.1617/s11527-021-01683-0</a></p>2022-11-22T21:18:36ZTextJournal contributioninfo:eu-repo/semantics/publishedVersiontextcontribution to journal10.1617/s11527-021-01683-0https://figshare.com/articles/journal_contribution/Influence_of_polymer_structure_and_amount_on_microstructure_and_properties_of_polyethylene-modified_asphalt_binders/21598560CC BY 4.0info:eu-repo/semantics/openAccessoai:figshare.com:article/215985602022-11-22T21:18:36Z
spellingShingle Influence of polymer structure and amount on microstructure and properties of polyethylene-modified asphalt binders
K. Lakshmi Roja (14159028)
Macromolecular and materials chemistry
Materials engineering
Mechanics of Materials
General Materials Science
Building and Construction
Civil and Structural Engineering
status_str publishedVersion
title Influence of polymer structure and amount on microstructure and properties of polyethylene-modified asphalt binders
title_full Influence of polymer structure and amount on microstructure and properties of polyethylene-modified asphalt binders
title_fullStr Influence of polymer structure and amount on microstructure and properties of polyethylene-modified asphalt binders
title_full_unstemmed Influence of polymer structure and amount on microstructure and properties of polyethylene-modified asphalt binders
title_short Influence of polymer structure and amount on microstructure and properties of polyethylene-modified asphalt binders
title_sort Influence of polymer structure and amount on microstructure and properties of polyethylene-modified asphalt binders
topic Macromolecular and materials chemistry
Materials engineering
Mechanics of Materials
General Materials Science
Building and Construction
Civil and Structural Engineering