Spatiotemporal variation of radionuclide dispersion from nuclear power plant accidents using FLEXPART mini-ensemble modeling

<p dir="ltr">Abstract. We investigate the spatiotemporal distribution of the radionuclides including iodine-131 (<sup>131</sup>I) and cesium-137 (<sup>137</sup>Cs), transported to Qatar from fictitious accidents at the upwind Barakah nuclear power plant (B-NPP...

وصف كامل

محفوظ في:
التفاصيل البيبلوغرافية
المؤلف الرئيسي: Seyed Omid Nabavi (19418872) (author)
مؤلفون آخرون: Theodoros Christoudias (8186838) (author), Yiannis Proestos (1806559) (author), Christos Fountoukis (4722963) (author), Huda Al-Sulaiti (17075197) (author), Jos Lelieveld (1806565) (author)
منشور في: 2023
الموضوعات:
الوسوم: إضافة وسم
لا توجد وسوم, كن أول من يضع وسما على هذه التسجيلة!
_version_ 1864513508124655616
author Seyed Omid Nabavi (19418872)
author2 Theodoros Christoudias (8186838)
Yiannis Proestos (1806559)
Christos Fountoukis (4722963)
Huda Al-Sulaiti (17075197)
Jos Lelieveld (1806565)
author2_role author
author
author
author
author
author_facet Seyed Omid Nabavi (19418872)
Theodoros Christoudias (8186838)
Yiannis Proestos (1806559)
Christos Fountoukis (4722963)
Huda Al-Sulaiti (17075197)
Jos Lelieveld (1806565)
author_role author
dc.creator.none.fl_str_mv Seyed Omid Nabavi (19418872)
Theodoros Christoudias (8186838)
Yiannis Proestos (1806559)
Christos Fountoukis (4722963)
Huda Al-Sulaiti (17075197)
Jos Lelieveld (1806565)
dc.date.none.fl_str_mv 2023-07-13T09:00:00Z
dc.identifier.none.fl_str_mv 10.5194/acp-23-7719-2023
dc.relation.none.fl_str_mv https://figshare.com/articles/journal_contribution/Spatiotemporal_variation_of_radionuclide_dispersion_from_nuclear_power_plant_accidents_using_FLEXPART_mini-ensemble_modeling/26644045
dc.rights.none.fl_str_mv CC BY 4.0
info:eu-repo/semantics/openAccess
dc.subject.none.fl_str_mv Earth sciences
Atmospheric sciences
Environmental sciences
Environmental biotechnology
Radionuclides
Sensitivity Analysis
Turbulence Schemes
Emission Profiles
Transport Modeling
Radiological Impact
Meteorological Data
dc.title.none.fl_str_mv Spatiotemporal variation of radionuclide dispersion from nuclear power plant accidents using FLEXPART mini-ensemble modeling
dc.type.none.fl_str_mv Text
Journal contribution
info:eu-repo/semantics/publishedVersion
text
contribution to journal
description <p dir="ltr">Abstract. We investigate the spatiotemporal distribution of the radionuclides including iodine-131 (<sup>131</sup>I) and cesium-137 (<sup>137</sup>Cs), transported to Qatar from fictitious accidents at the upwind Barakah nuclear power plant (B-NPP) in the United Arab Emirates (UAE). To model the dispersion of radionuclides, we use the Lagrangian particle–air parcel dispersion model FLEXible PARTicle (FLEXPART) and FLEXPART coupled with the Weather Research and Forecasting model (FLEXPART–WRF). A four-member mini-ensemble of meteorological inputs is used to investigate the impact of meteorological inputs on the radionuclide dispersion modeling. The mini-ensemble includes one forecast dataset (Global Forecast System, GFS) and three (re)analysis datasets (native-resolution and downscaled NCEP final analysis – FNL, as well as downscaled ERA5). Additionally, we explore the sensitivity of the radionuclide dispersion simulations to variations in the turbulence schemes, as well as the temporal and vertical emission profiles, and the location of emission sources. According to the simulated age spectrum of the Lagrangian particles, radionuclides enter southern Qatar about 20 to 30 h after release. Most of the radionuclide deposition in the study area occurs within 80 h after release. The most populated areas of Qatar coincide with moderate <sup>131</sup>I concentrations and <sup>137</sup>Cs deposition, while uninhabited areas in southern Qatar receive the highest amounts. A larger number of long-lived particles is found in the FNL-based simulations, which is interpreted as a greater dispersion of particles at a greater distance from the emission location. The highest simulated <sup>131</sup>I and <sup>137</sup>Cs deposition shows a pronounced spatiotemporal pattern. The largest impacts are found in the south and southeast of Qatar, during the early daytime development of the boundary layer, and during the cold period of the year. The results show remarkable differences in the spatiotemporal distribution of <sup>131</sup>I and <sup>137</sup>Cs simulations based on the FNL and GFS datasets, which share a common base meteorological model. As part of a sensitivity analysis involving different model setups, changing the emission point from B-NPP to Bushehr NPP (Bu-NPP) results in a reduced transfer of radioactive materials to Qatar, except in the spring season. Bu-NPP simulations reveal distinct spatial patterns, with peak<sup> 131</sup>I concentrations and <sup>137</sup>Cs deposition observed in northern and eastern Qatar during winter and spring.</p><h2>Other Information</h2><p dir="ltr">Published in: Atmospheric Chemistry and Physics<br>License: <a href="https://creativecommons.org/licenses/by/4.0/" target="_blank">https://creativecommons.org/licenses/by/4.0/</a><br>See article on publisher's website: <a href="https://dx.doi.org/10.5194/acp-23-7719-2023" target="_blank">https://dx.doi.org/10.5194/acp-23-7719-2023</a></p>
eu_rights_str_mv openAccess
id Manara2_cb1cbd85d1c392fb65b73988da95331f
identifier_str_mv 10.5194/acp-23-7719-2023
network_acronym_str Manara2
network_name_str Manara2
oai_identifier_str oai:figshare.com:article/26644045
publishDate 2023
repository.mail.fl_str_mv
repository.name.fl_str_mv
repository_id_str
rights_invalid_str_mv CC BY 4.0
spelling Spatiotemporal variation of radionuclide dispersion from nuclear power plant accidents using FLEXPART mini-ensemble modelingSeyed Omid Nabavi (19418872)Theodoros Christoudias (8186838)Yiannis Proestos (1806559)Christos Fountoukis (4722963)Huda Al-Sulaiti (17075197)Jos Lelieveld (1806565)Earth sciencesAtmospheric sciencesEnvironmental sciencesEnvironmental biotechnologyRadionuclidesSensitivity AnalysisTurbulence SchemesEmission ProfilesTransport ModelingRadiological ImpactMeteorological Data<p dir="ltr">Abstract. We investigate the spatiotemporal distribution of the radionuclides including iodine-131 (<sup>131</sup>I) and cesium-137 (<sup>137</sup>Cs), transported to Qatar from fictitious accidents at the upwind Barakah nuclear power plant (B-NPP) in the United Arab Emirates (UAE). To model the dispersion of radionuclides, we use the Lagrangian particle–air parcel dispersion model FLEXible PARTicle (FLEXPART) and FLEXPART coupled with the Weather Research and Forecasting model (FLEXPART–WRF). A four-member mini-ensemble of meteorological inputs is used to investigate the impact of meteorological inputs on the radionuclide dispersion modeling. The mini-ensemble includes one forecast dataset (Global Forecast System, GFS) and three (re)analysis datasets (native-resolution and downscaled NCEP final analysis – FNL, as well as downscaled ERA5). Additionally, we explore the sensitivity of the radionuclide dispersion simulations to variations in the turbulence schemes, as well as the temporal and vertical emission profiles, and the location of emission sources. According to the simulated age spectrum of the Lagrangian particles, radionuclides enter southern Qatar about 20 to 30 h after release. Most of the radionuclide deposition in the study area occurs within 80 h after release. The most populated areas of Qatar coincide with moderate <sup>131</sup>I concentrations and <sup>137</sup>Cs deposition, while uninhabited areas in southern Qatar receive the highest amounts. A larger number of long-lived particles is found in the FNL-based simulations, which is interpreted as a greater dispersion of particles at a greater distance from the emission location. The highest simulated <sup>131</sup>I and <sup>137</sup>Cs deposition shows a pronounced spatiotemporal pattern. The largest impacts are found in the south and southeast of Qatar, during the early daytime development of the boundary layer, and during the cold period of the year. The results show remarkable differences in the spatiotemporal distribution of <sup>131</sup>I and <sup>137</sup>Cs simulations based on the FNL and GFS datasets, which share a common base meteorological model. As part of a sensitivity analysis involving different model setups, changing the emission point from B-NPP to Bushehr NPP (Bu-NPP) results in a reduced transfer of radioactive materials to Qatar, except in the spring season. Bu-NPP simulations reveal distinct spatial patterns, with peak<sup> 131</sup>I concentrations and <sup>137</sup>Cs deposition observed in northern and eastern Qatar during winter and spring.</p><h2>Other Information</h2><p dir="ltr">Published in: Atmospheric Chemistry and Physics<br>License: <a href="https://creativecommons.org/licenses/by/4.0/" target="_blank">https://creativecommons.org/licenses/by/4.0/</a><br>See article on publisher's website: <a href="https://dx.doi.org/10.5194/acp-23-7719-2023" target="_blank">https://dx.doi.org/10.5194/acp-23-7719-2023</a></p>2023-07-13T09:00:00ZTextJournal contributioninfo:eu-repo/semantics/publishedVersiontextcontribution to journal10.5194/acp-23-7719-2023https://figshare.com/articles/journal_contribution/Spatiotemporal_variation_of_radionuclide_dispersion_from_nuclear_power_plant_accidents_using_FLEXPART_mini-ensemble_modeling/26644045CC BY 4.0info:eu-repo/semantics/openAccessoai:figshare.com:article/266440452023-07-13T09:00:00Z
spellingShingle Spatiotemporal variation of radionuclide dispersion from nuclear power plant accidents using FLEXPART mini-ensemble modeling
Seyed Omid Nabavi (19418872)
Earth sciences
Atmospheric sciences
Environmental sciences
Environmental biotechnology
Radionuclides
Sensitivity Analysis
Turbulence Schemes
Emission Profiles
Transport Modeling
Radiological Impact
Meteorological Data
status_str publishedVersion
title Spatiotemporal variation of radionuclide dispersion from nuclear power plant accidents using FLEXPART mini-ensemble modeling
title_full Spatiotemporal variation of radionuclide dispersion from nuclear power plant accidents using FLEXPART mini-ensemble modeling
title_fullStr Spatiotemporal variation of radionuclide dispersion from nuclear power plant accidents using FLEXPART mini-ensemble modeling
title_full_unstemmed Spatiotemporal variation of radionuclide dispersion from nuclear power plant accidents using FLEXPART mini-ensemble modeling
title_short Spatiotemporal variation of radionuclide dispersion from nuclear power plant accidents using FLEXPART mini-ensemble modeling
title_sort Spatiotemporal variation of radionuclide dispersion from nuclear power plant accidents using FLEXPART mini-ensemble modeling
topic Earth sciences
Atmospheric sciences
Environmental sciences
Environmental biotechnology
Radionuclides
Sensitivity Analysis
Turbulence Schemes
Emission Profiles
Transport Modeling
Radiological Impact
Meteorological Data