Self-assembly of Pseudo-Dipolar Nanoparticles at Low Densities and Strong Coupling

<p dir="ltr">Nanocolloids having directional interactions are highly relevant for designing new self-assembled materials easy to control. In this article we report stochastic dynamics simulations of finite-size pseudo-dipolar colloids immersed in an implicit dielectric solvent using...

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محفوظ في:
التفاصيل البيبلوغرافية
المؤلف الرئيسي: Mariano E. Brito (18622741) (author)
مؤلفون آخرون: Marcelo A. Carignano (1546291) (author), Verónica I. Marconi (18622744) (author)
منشور في: 2020
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author Mariano E. Brito (18622741)
author2 Marcelo A. Carignano (1546291)
Verónica I. Marconi (18622744)
author2_role author
author
author_facet Mariano E. Brito (18622741)
Marcelo A. Carignano (1546291)
Verónica I. Marconi (18622744)
author_role author
dc.creator.none.fl_str_mv Mariano E. Brito (18622741)
Marcelo A. Carignano (1546291)
Verónica I. Marconi (18622744)
dc.date.none.fl_str_mv 2020-12-01T06:00:00Z
dc.identifier.none.fl_str_mv 10.1038/s41598-020-60417-4
dc.relation.none.fl_str_mv https://figshare.com/articles/journal_contribution/Self-assembly_of_Pseudo-Dipolar_Nanoparticles_at_Low_Densities_and_Strong_Coupling/25911172
dc.rights.none.fl_str_mv CC BY 4.0
info:eu-repo/semantics/openAccess
dc.subject.none.fl_str_mv Chemical sciences
Macromolecular and materials chemistry
Physical chemistry
Engineering
Materials engineering
Nanotechnology
Antiparallel alignment
Colloids
Coulombic interaction
Dynamically-arrested
Finite-size
Nanocolloids
Self-assembly
Simulations
String-fluid
String-gel
Structural characterization
Thermal energy
dc.title.none.fl_str_mv Self-assembly of Pseudo-Dipolar Nanoparticles at Low Densities and Strong Coupling
dc.type.none.fl_str_mv Text
Journal contribution
info:eu-repo/semantics/publishedVersion
text
contribution to journal
description <p dir="ltr">Nanocolloids having directional interactions are highly relevant for designing new self-assembled materials easy to control. In this article we report stochastic dynamics simulations of finite-size pseudo-dipolar colloids immersed in an implicit dielectric solvent using a realistic continuous description of the quasi-hard Coulombic interaction. We investigate structural and dynamical properties near the low-temperature and highly-diluted limits. This system self-assembles in a rich variety of string-like configurations, depicting three clearly distinguishable regimes with decreasing temperature: fluid, composed by isolated colloids; string-fluid, a gas of short string-like clusters; and string-gel, a percolated network. By structural characterization using radial distribution functions and cluster properties, we calculate the state diagram, verifying the presence of string-fluid regime. Regarding the string-gel regime, we show that the antiparallel alignment of the network chains arises as a novel self-assembly mechanism when the characteristic interaction energy exceeds the thermal energy in two orders of magnitude, ud/kBT ≈ 100. This is associated to relevant structural modifications in the network connectivity and porosity. Furthermore, our results give insights about the dynamically-arrested nature of the string-gel regime, where we show that the slow relaxation takes place in minuscule energy steps that reflect local rearrangements of the network.</p><h2>Other Information</h2><p dir="ltr">Published in: Scientific Reports<br>License: <a href="https://creativecommons.org/licenses/by/4.0" target="_blank">https://creativecommons.org/licenses/by/4.0</a><br>See article on publisher's website: <a href="https://dx.doi.org/10.1038/s41598-020-60417-4" target="_blank">https://dx.doi.org/10.1038/s41598-020-60417-4</a></p>
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identifier_str_mv 10.1038/s41598-020-60417-4
network_acronym_str Manara2
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oai_identifier_str oai:figshare.com:article/25911172
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spelling Self-assembly of Pseudo-Dipolar Nanoparticles at Low Densities and Strong CouplingMariano E. Brito (18622741)Marcelo A. Carignano (1546291)Verónica I. Marconi (18622744)Chemical sciencesMacromolecular and materials chemistryPhysical chemistryEngineeringMaterials engineeringNanotechnologyAntiparallel alignmentColloidsCoulombic interactionDynamically-arrestedFinite-sizeNanocolloidsSelf-assemblySimulationsString-fluidString-gelStructural characterizationThermal energy<p dir="ltr">Nanocolloids having directional interactions are highly relevant for designing new self-assembled materials easy to control. In this article we report stochastic dynamics simulations of finite-size pseudo-dipolar colloids immersed in an implicit dielectric solvent using a realistic continuous description of the quasi-hard Coulombic interaction. We investigate structural and dynamical properties near the low-temperature and highly-diluted limits. This system self-assembles in a rich variety of string-like configurations, depicting three clearly distinguishable regimes with decreasing temperature: fluid, composed by isolated colloids; string-fluid, a gas of short string-like clusters; and string-gel, a percolated network. By structural characterization using radial distribution functions and cluster properties, we calculate the state diagram, verifying the presence of string-fluid regime. Regarding the string-gel regime, we show that the antiparallel alignment of the network chains arises as a novel self-assembly mechanism when the characteristic interaction energy exceeds the thermal energy in two orders of magnitude, ud/kBT ≈ 100. This is associated to relevant structural modifications in the network connectivity and porosity. Furthermore, our results give insights about the dynamically-arrested nature of the string-gel regime, where we show that the slow relaxation takes place in minuscule energy steps that reflect local rearrangements of the network.</p><h2>Other Information</h2><p dir="ltr">Published in: Scientific Reports<br>License: <a href="https://creativecommons.org/licenses/by/4.0" target="_blank">https://creativecommons.org/licenses/by/4.0</a><br>See article on publisher's website: <a href="https://dx.doi.org/10.1038/s41598-020-60417-4" target="_blank">https://dx.doi.org/10.1038/s41598-020-60417-4</a></p>2020-12-01T06:00:00ZTextJournal contributioninfo:eu-repo/semantics/publishedVersiontextcontribution to journal10.1038/s41598-020-60417-4https://figshare.com/articles/journal_contribution/Self-assembly_of_Pseudo-Dipolar_Nanoparticles_at_Low_Densities_and_Strong_Coupling/25911172CC BY 4.0info:eu-repo/semantics/openAccessoai:figshare.com:article/259111722020-12-01T06:00:00Z
spellingShingle Self-assembly of Pseudo-Dipolar Nanoparticles at Low Densities and Strong Coupling
Mariano E. Brito (18622741)
Chemical sciences
Macromolecular and materials chemistry
Physical chemistry
Engineering
Materials engineering
Nanotechnology
Antiparallel alignment
Colloids
Coulombic interaction
Dynamically-arrested
Finite-size
Nanocolloids
Self-assembly
Simulations
String-fluid
String-gel
Structural characterization
Thermal energy
status_str publishedVersion
title Self-assembly of Pseudo-Dipolar Nanoparticles at Low Densities and Strong Coupling
title_full Self-assembly of Pseudo-Dipolar Nanoparticles at Low Densities and Strong Coupling
title_fullStr Self-assembly of Pseudo-Dipolar Nanoparticles at Low Densities and Strong Coupling
title_full_unstemmed Self-assembly of Pseudo-Dipolar Nanoparticles at Low Densities and Strong Coupling
title_short Self-assembly of Pseudo-Dipolar Nanoparticles at Low Densities and Strong Coupling
title_sort Self-assembly of Pseudo-Dipolar Nanoparticles at Low Densities and Strong Coupling
topic Chemical sciences
Macromolecular and materials chemistry
Physical chemistry
Engineering
Materials engineering
Nanotechnology
Antiparallel alignment
Colloids
Coulombic interaction
Dynamically-arrested
Finite-size
Nanocolloids
Self-assembly
Simulations
String-fluid
String-gel
Structural characterization
Thermal energy