Rational Optimization of Ammonium and Phosphonium Cations of Bifunctional Organoborane Catalysts for Copolymerization of Propylene Oxide with CO<sub>2</sub> to Afford Poly(propylene carbonate)

Rational Optimization of Ammonium and Phosphonium Cations of Bifunctional Organoborane Catalysts for Copolymerization of Propylene Oxide with CO<sub>2</sub> to Afford Poly(propylene carbonate)

Ring-opening copolymerization (ROCOP) of CO<sub>2</sub> and propylene oxide (PO) is a challenging task due to its tendency to generate a polyether linkage and cyclic carbonate. Our group recently reported a series of mononuclear organoborane catalysts for the efficient ROCOP of CO<sub...

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التفاصيل البيبلوغرافية
المؤلف الرئيسي:	Cheng-Kai Xu (10150998) (author)
مؤلفون آخرون:	Chenjie Lu (3897784) (author), Shuo Zhao (1545043) (author), Guan-Wen Yang (1879624) (author), Wei Li (7081) (author), Jingdai Wang (1622767) (author), Guang-Peng Wu (1495657) (author)
منشور في:	2024
الموضوعات:	Biochemistry Microbiology Biotechnology Evolutionary Biology Cancer Space Science Environmental Sciences not elsewhere classified Chemical Sciences not elsewhere classified stronger lewis acidity group recently reported facilitate chain propagation exhibited inferior performance challenging task due catalyst molecule imparted backbiting side reaction optimal catalytic performance mononuclear organoborane catalysts catalysts bearing alfa bifunctional organoborane catalysts superior catalytic activity cyclohexene oxide (< β </ sup α </ sup 31 </ sup ammonium counterparts stems 3 </ sub 2 </ sub h (< sup catalytic activity n </ 59 </ 142 </ propylene oxide sup >< ></ sup catalysts featuring advanced catalysts po (< therefore proposed successfully realized soc .,</ propylene carbonate produce poly previous borinane polyether linkage indispensable role h atom ed .</ dominated interaction cyclic carbonate cationic part cation without afford poly
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مواد مشابهة

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