Adaptive dry adhesives with tunable morphology via shape memory elastomeric bilayers

<p>Dry adhesives offer appealing advantages such as reusability and clean detachment, yet their performance is fundamentally constrained by the trade-off between adhesion strength and fracture toughness. In this work, we present adaptive bilayer dry adhesives that integrate a thin, compliant e...

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Autor principal: Junhyung Kim (1277919) (author)
Outros Autores: Wooyoung Kim (2390494) (author), Seok Kim (1718575) (author)
Publicado em: 2025
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author Junhyung Kim (1277919)
author2 Wooyoung Kim (2390494)
Seok Kim (1718575)
author2_role author
author
author_facet Junhyung Kim (1277919)
Wooyoung Kim (2390494)
Seok Kim (1718575)
author_role author
dc.creator.none.fl_str_mv Junhyung Kim (1277919)
Wooyoung Kim (2390494)
Seok Kim (1718575)
dc.date.none.fl_str_mv 2025-11-25T18:00:15Z
dc.identifier.none.fl_str_mv 10.6084/m9.figshare.30713088.v1
dc.relation.none.fl_str_mv https://figshare.com/articles/dataset/Adaptive_dry_adhesives_with_tunable_morphology_via_shape_memory_elastomeric_bilayers/30713088
dc.rights.none.fl_str_mv CC BY 4.0
info:eu-repo/semantics/openAccess
dc.subject.none.fl_str_mv Biophysics
Cell Biology
Biotechnology
Computational Biology
Space Science
Environmental Sciences not elsewhere classified
Biological Sciences not elsewhere classified
Chemical Sciences not elsewhere classified
Physical Sciences not elsewhere classified
Information Systems not elsewhere classified
Shape memory polymers
dry adhesives
bilayer architectures
heterogeneous structures
dc.title.none.fl_str_mv Adaptive dry adhesives with tunable morphology via shape memory elastomeric bilayers
dc.type.none.fl_str_mv Dataset
info:eu-repo/semantics/publishedVersion
dataset
description <p>Dry adhesives offer appealing advantages such as reusability and clean detachment, yet their performance is fundamentally constrained by the trade-off between adhesion strength and fracture toughness. In this work, we present adaptive bilayer dry adhesives that integrate a thin, compliant elastomeric polydimethylsiloxane (PDMS) surface with a stiff shape memory polymer (SMP) backing layer. While the SMP layer enables shape programming through its rubber-to-glass transition, the PDMS layer suppresses catastrophic adhesive failure and preserves adhesion. Finite element analysis results reveal that the programmed bilayer surface forms extensive interfacial contact with minimal preload, outperforming conventional elastomeric adhesives. Adhesion tests further demonstrate that the bilayer achieves nearly ten-fold higher adhesion compared to PDMS, while maintaining greater detachment toughness relative to SMP, thereby alleviating the inherent trade-off. Moreover, the bilayer’s shape programming capability enables stable and repeatable adhesion to curved surfaces without requiring additional rubber-to-glass transitions. For practical demonstrations, we fabricated an integrated heater-assisted adhesive hook capable of supporting a 2 kg load on diverse wall surfaces, with reversible and reusable operation. This bilayer adhesive strategy provides a generalized design principle to overcome the incompatibility between adhesion and toughness, offering strong potential for applications in soft robotics, wearable systems, and transfer printing.</p>
eu_rights_str_mv openAccess
id Manara_3f790c2602bdcad59cf054f70f1f03ce
identifier_str_mv 10.6084/m9.figshare.30713088.v1
network_acronym_str Manara
network_name_str ManaraRepo
oai_identifier_str oai:figshare.com:article/30713088
publishDate 2025
repository.mail.fl_str_mv
repository.name.fl_str_mv
repository_id_str
rights_invalid_str_mv CC BY 4.0
spelling Adaptive dry adhesives with tunable morphology via shape memory elastomeric bilayersJunhyung Kim (1277919)Wooyoung Kim (2390494)Seok Kim (1718575)BiophysicsCell BiologyBiotechnologyComputational BiologySpace ScienceEnvironmental Sciences not elsewhere classifiedBiological Sciences not elsewhere classifiedChemical Sciences not elsewhere classifiedPhysical Sciences not elsewhere classifiedInformation Systems not elsewhere classifiedShape memory polymersdry adhesivesbilayer architecturesheterogeneous structures<p>Dry adhesives offer appealing advantages such as reusability and clean detachment, yet their performance is fundamentally constrained by the trade-off between adhesion strength and fracture toughness. In this work, we present adaptive bilayer dry adhesives that integrate a thin, compliant elastomeric polydimethylsiloxane (PDMS) surface with a stiff shape memory polymer (SMP) backing layer. While the SMP layer enables shape programming through its rubber-to-glass transition, the PDMS layer suppresses catastrophic adhesive failure and preserves adhesion. Finite element analysis results reveal that the programmed bilayer surface forms extensive interfacial contact with minimal preload, outperforming conventional elastomeric adhesives. Adhesion tests further demonstrate that the bilayer achieves nearly ten-fold higher adhesion compared to PDMS, while maintaining greater detachment toughness relative to SMP, thereby alleviating the inherent trade-off. Moreover, the bilayer’s shape programming capability enables stable and repeatable adhesion to curved surfaces without requiring additional rubber-to-glass transitions. For practical demonstrations, we fabricated an integrated heater-assisted adhesive hook capable of supporting a 2 kg load on diverse wall surfaces, with reversible and reusable operation. This bilayer adhesive strategy provides a generalized design principle to overcome the incompatibility between adhesion and toughness, offering strong potential for applications in soft robotics, wearable systems, and transfer printing.</p>2025-11-25T18:00:15ZDatasetinfo:eu-repo/semantics/publishedVersiondataset10.6084/m9.figshare.30713088.v1https://figshare.com/articles/dataset/Adaptive_dry_adhesives_with_tunable_morphology_via_shape_memory_elastomeric_bilayers/30713088CC BY 4.0info:eu-repo/semantics/openAccessoai:figshare.com:article/307130882025-11-25T18:00:15Z
spellingShingle Adaptive dry adhesives with tunable morphology via shape memory elastomeric bilayers
Junhyung Kim (1277919)
Biophysics
Cell Biology
Biotechnology
Computational Biology
Space Science
Environmental Sciences not elsewhere classified
Biological Sciences not elsewhere classified
Chemical Sciences not elsewhere classified
Physical Sciences not elsewhere classified
Information Systems not elsewhere classified
Shape memory polymers
dry adhesives
bilayer architectures
heterogeneous structures
status_str publishedVersion
title Adaptive dry adhesives with tunable morphology via shape memory elastomeric bilayers
title_full Adaptive dry adhesives with tunable morphology via shape memory elastomeric bilayers
title_fullStr Adaptive dry adhesives with tunable morphology via shape memory elastomeric bilayers
title_full_unstemmed Adaptive dry adhesives with tunable morphology via shape memory elastomeric bilayers
title_short Adaptive dry adhesives with tunable morphology via shape memory elastomeric bilayers
title_sort Adaptive dry adhesives with tunable morphology via shape memory elastomeric bilayers
topic Biophysics
Cell Biology
Biotechnology
Computational Biology
Space Science
Environmental Sciences not elsewhere classified
Biological Sciences not elsewhere classified
Chemical Sciences not elsewhere classified
Physical Sciences not elsewhere classified
Information Systems not elsewhere classified
Shape memory polymers
dry adhesives
bilayer architectures
heterogeneous structures