Greening Fine Chemical Production via Continuous Flow Technology: An LCA-TEA-SA Integrated Assessment of <i>p</i>‑Nitrobenzoic Acid

The fine chemical industry is reevaluating its traditional manufacturing paradigms, moving toward greener, safer processes and cost-effective practices. Continuous flow technology (CFT) stands out among emerging methodologies due to its superior performance and significant commercial potential, but...

وصف كامل

محفوظ في:
التفاصيل البيبلوغرافية
المؤلف الرئيسي: Chen Feng (298683) (author)
مؤلفون آخرون: Ran An (456243) (author), Hao Xiao (43530) (author), Tianshu Ji (11654096) (author), Yacong Hu (22656820) (author), Kun Yan (300887) (author), Kailingli Liao (6110129) (author), Hanbo Gao (13222626) (author), Zhidong Xu (1834) (author), Jinping Tian (1496839) (author), Lyujun Chen (13222632) (author)
منشور في: 2025
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الوصف
الملخص:The fine chemical industry is reevaluating its traditional manufacturing paradigms, moving toward greener, safer processes and cost-effective practices. Continuous flow technology (CFT) stands out among emerging methodologies due to its superior performance and significant commercial potential, but it still lacks comprehensive environment-economy-safety trade-off assessments and the exploration of optimal scale-up pathways. To address the gap, we developed a model by integrating green chemistry efficiency assessments, life cycle environment-economy-safety evaluations, and scale effects. The model was employed to the oxidation of <i>p</i>-nitrotoluene to <i>p</i>-nitrobenzoic acid based on commercialized-scale production. We assessed the traditional batch-wise technology (BWT) and emerging continuous flow technology to elucidate the environment-economy-safety trade-off and scale effects. The key findings include the following: (1) CFT outperformed BWT with a 16.91% reduction in 100 year global warming potential, a 13.73% decrease in capital and operating expense, and a 1.5% improvement in overall safety score under real production conditions. (2) A trade-off model identified 154–160 °C as an optimal window where CFT excelled in environment-economy-temperature safety performance. As temperature rose, CFT showed decreasing unit emissions and cost. (3) At scales above 2385 tons/year, CFT could become more cost-effective than BWT. CFT consistently outperforms BWT across all production scales in terms of both environmental performance and economic scalability. The volumetric expansion of BWT proved to be a more sustainable scale-up route than numbering-up. This study can offer insights into the transformation toward sustainable fine chemical production practices.