Dimolybdenum Paddlewheel Complexes with Cation Binding Sites as Electrolyte Additives to Manipulate the Solid-Electrolyte Interphase at Lithium Metal Anodes

The use of electrolyte additives at millimolar loadings to control the surface chemistry of lithium metal anodes (LMAs) is a leading strategy to improve lithium metal batteries and promote electrosynthetic reactions. Whereas previous studies employed either inorganic or organic additives, in this st...

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Bibliographic Details
Main Author:	Simon G. Gersib (21432741) (author)
Other Authors:	Erik J. Askins (10182245) (author), Matthew Li (743636) (author), S. M. Supundrika Subasinghe (15197638) (author), Biki Kumar Behera (21432744) (author), Dan McElheny (249371) (author), Seoung-Bum Son (1586413) (author), Khalil Amine (1329924) (author), Ksenija D. Glusac (1633834) (author), Neal P. Mankad (1474654) (author)
Published:	2025
Subjects:	Biophysics Biochemistry Space Science Biological Sciences not elsewhere classified Chemical Sciences not elsewhere classified sup >+</ sup promote electrosynthetic reactions parasitic side reactions lithium metal anodes g ., overpotential dimolybdenum paddlewheel complexes dimolybdenum paddlewheel complex coulombic efficiency ), cationically charged aggregates calendar aging tests 2 -( 2 promote reversible li li plating properties li plating conditions second coordination sphere first organometallic additive cation binding sites 4 </ sub 1 </ b solid electrolyte interphase electrolyte interphase organometallic synthesis additive protects electrolyte additives surface structure surface chemistry products thereof produce modest organic additives notable benefit modified sei millimolar loadings measurable improvements leading strategy induces immobilization data disclose acetate ], [< b
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Dimolybdenum Paddlewheel Complexes with Cation Binding Sites as Electrolyte Additives to Manipulate the Solid-Electrolyte Interphase at Lithium Metal Anodes

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