Green synthesized nano-TiO<sub>2</sub> from Tamarindusindica leaf extract for photo-degradation of combination of dyes by suspension and immobilization on inert supports

<p>The present study aims to use green synthesized TiO<sub>2</sub> as a photocatalyst in suspended and immobilized form under UV light to efficiently degrade a combination of reactive dyes, namely titan yellow, methyl orange, rhodamine B, and methylene blue. TiO<sub>2</sub...

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Main Author: Shilpa Hiremath (20101953) (author)
Other Authors: Sudeep Mudhulu (20101956) (author), C. Vidya (20101959) (author), M. N. Chandraprabha (20101962) (author), Vinutha Moses (20101965) (author), C. Manjunatha (5147057) (author)
Published: 2024
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_version_ 1852025464489508864
author Shilpa Hiremath (20101953)
author2 Sudeep Mudhulu (20101956)
C. Vidya (20101959)
M. N. Chandraprabha (20101962)
Vinutha Moses (20101965)
C. Manjunatha (5147057)
author2_role author
author
author
author
author
author_facet Shilpa Hiremath (20101953)
Sudeep Mudhulu (20101956)
C. Vidya (20101959)
M. N. Chandraprabha (20101962)
Vinutha Moses (20101965)
C. Manjunatha (5147057)
author_role author
dc.creator.none.fl_str_mv Shilpa Hiremath (20101953)
Sudeep Mudhulu (20101956)
C. Vidya (20101959)
M. N. Chandraprabha (20101962)
Vinutha Moses (20101965)
C. Manjunatha (5147057)
dc.date.none.fl_str_mv 2024-11-03T22:40:12Z
dc.identifier.none.fl_str_mv 10.6084/m9.figshare.27600372.v1
dc.relation.none.fl_str_mv https://figshare.com/articles/online_resource/Green_synthesized_nano-TiO_sub_2_sub_from_Tamarindusindica_leaf_extract_for_photo-degradation_of_combination_of_dyes_by_suspension_and_immobilization_on_inert_supports/27600372
dc.rights.none.fl_str_mv CC BY 4.0
info:eu-repo/semantics/openAccess
dc.subject.none.fl_str_mv Biochemistry
Medicine
Molecular Biology
Biotechnology
Developmental Biology
Cancer
Inorganic Chemistry
Biological Sciences not elsewhere classified
Chemical Sciences not elsewhere classified
Nano TiO2
immobilization
photodegradation
mixture of dyes
continuous mode
dc.title.none.fl_str_mv Green synthesized nano-TiO<sub>2</sub> from Tamarindusindica leaf extract for photo-degradation of combination of dyes by suspension and immobilization on inert supports
dc.type.none.fl_str_mv Text
Online resource
info:eu-repo/semantics/publishedVersion
text
description <p>The present study aims to use green synthesized TiO<sub>2</sub> as a photocatalyst in suspended and immobilized form under UV light to efficiently degrade a combination of reactive dyes, namely titan yellow, methyl orange, rhodamine B, and methylene blue. TiO<sub>2</sub> nanoparticles (NPs) were synthesized using <i>Tamarindus indica</i> leaf extract and were utilized to parametrically study photo-degradation at room temperature. The green synthesized NPs were characterized by Powder XRD, SEM, and FTIR techniques to understand the crystalline phase/purity, morphology, and functional groups respectively. The TiO<sub>2</sub> in suspension under UV light showed >90% degradation towards a 10 ppm composite dye at a loading of 1.5 gL<sup>−1</sup>, pH 7, and an irradiation time of 120 min. Subsequently, TiO<sub>2</sub> was further immobilized in-situ, on inert supports of perlite granules and glass and studied for catalytic activity in batch and continuous modes. The TiO<sub>2</sub> nanoparticles immobilized on perlite granules and glass showed 59 and 48% degradation in batch operation under the same conditions as in suspended form. In continuous mode, the highest degradation activity was recorded at 2 Lh<sup>−1</sup> after 4 passes. Further, kinetic studies reveal that the degradation reaction is best described by Langmuir Hinshelwood kinetics for both suspended and immobilized TiO<sub>2</sub>.</p>
eu_rights_str_mv openAccess
id Manara_87fc28282024940780256b0ec54e3b86
identifier_str_mv 10.6084/m9.figshare.27600372.v1
network_acronym_str Manara
network_name_str ManaraRepo
oai_identifier_str oai:figshare.com:article/27600372
publishDate 2024
repository.mail.fl_str_mv
repository.name.fl_str_mv
repository_id_str
rights_invalid_str_mv CC BY 4.0
spelling Green synthesized nano-TiO<sub>2</sub> from Tamarindusindica leaf extract for photo-degradation of combination of dyes by suspension and immobilization on inert supportsShilpa Hiremath (20101953)Sudeep Mudhulu (20101956)C. Vidya (20101959)M. N. Chandraprabha (20101962)Vinutha Moses (20101965)C. Manjunatha (5147057)BiochemistryMedicineMolecular BiologyBiotechnologyDevelopmental BiologyCancerInorganic ChemistryBiological Sciences not elsewhere classifiedChemical Sciences not elsewhere classifiedNano TiO2immobilizationphotodegradationmixture of dyescontinuous mode<p>The present study aims to use green synthesized TiO<sub>2</sub> as a photocatalyst in suspended and immobilized form under UV light to efficiently degrade a combination of reactive dyes, namely titan yellow, methyl orange, rhodamine B, and methylene blue. TiO<sub>2</sub> nanoparticles (NPs) were synthesized using <i>Tamarindus indica</i> leaf extract and were utilized to parametrically study photo-degradation at room temperature. The green synthesized NPs were characterized by Powder XRD, SEM, and FTIR techniques to understand the crystalline phase/purity, morphology, and functional groups respectively. The TiO<sub>2</sub> in suspension under UV light showed >90% degradation towards a 10 ppm composite dye at a loading of 1.5 gL<sup>−1</sup>, pH 7, and an irradiation time of 120 min. Subsequently, TiO<sub>2</sub> was further immobilized in-situ, on inert supports of perlite granules and glass and studied for catalytic activity in batch and continuous modes. The TiO<sub>2</sub> nanoparticles immobilized on perlite granules and glass showed 59 and 48% degradation in batch operation under the same conditions as in suspended form. In continuous mode, the highest degradation activity was recorded at 2 Lh<sup>−1</sup> after 4 passes. Further, kinetic studies reveal that the degradation reaction is best described by Langmuir Hinshelwood kinetics for both suspended and immobilized TiO<sub>2</sub>.</p>2024-11-03T22:40:12ZTextOnline resourceinfo:eu-repo/semantics/publishedVersiontext10.6084/m9.figshare.27600372.v1https://figshare.com/articles/online_resource/Green_synthesized_nano-TiO_sub_2_sub_from_Tamarindusindica_leaf_extract_for_photo-degradation_of_combination_of_dyes_by_suspension_and_immobilization_on_inert_supports/27600372CC BY 4.0info:eu-repo/semantics/openAccessoai:figshare.com:article/276003722024-11-03T22:40:12Z
spellingShingle Green synthesized nano-TiO<sub>2</sub> from Tamarindusindica leaf extract for photo-degradation of combination of dyes by suspension and immobilization on inert supports
Shilpa Hiremath (20101953)
Biochemistry
Medicine
Molecular Biology
Biotechnology
Developmental Biology
Cancer
Inorganic Chemistry
Biological Sciences not elsewhere classified
Chemical Sciences not elsewhere classified
Nano TiO2
immobilization
photodegradation
mixture of dyes
continuous mode
status_str publishedVersion
title Green synthesized nano-TiO<sub>2</sub> from Tamarindusindica leaf extract for photo-degradation of combination of dyes by suspension and immobilization on inert supports
title_full Green synthesized nano-TiO<sub>2</sub> from Tamarindusindica leaf extract for photo-degradation of combination of dyes by suspension and immobilization on inert supports
title_fullStr Green synthesized nano-TiO<sub>2</sub> from Tamarindusindica leaf extract for photo-degradation of combination of dyes by suspension and immobilization on inert supports
title_full_unstemmed Green synthesized nano-TiO<sub>2</sub> from Tamarindusindica leaf extract for photo-degradation of combination of dyes by suspension and immobilization on inert supports
title_short Green synthesized nano-TiO<sub>2</sub> from Tamarindusindica leaf extract for photo-degradation of combination of dyes by suspension and immobilization on inert supports
title_sort Green synthesized nano-TiO<sub>2</sub> from Tamarindusindica leaf extract for photo-degradation of combination of dyes by suspension and immobilization on inert supports
topic Biochemistry
Medicine
Molecular Biology
Biotechnology
Developmental Biology
Cancer
Inorganic Chemistry
Biological Sciences not elsewhere classified
Chemical Sciences not elsewhere classified
Nano TiO2
immobilization
photodegradation
mixture of dyes
continuous mode