Assembling a Metastable Electron Fence within Gold-Zeolite Interfaces for Boosted Propylene Epoxidation

Selective oxidation of hydrocarbons represents a cornerstone reaction in the chemical industry, yet achieving both high activity and selectivity remains challenging. Gold catalysts, renowned for their resistance to overoxidation, are hindered by poor oxygen activation. Here, we develop an “electron...

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Bibliographic Details
Main Author:	Qianhong Wang (14497105) (author)
Other Authors:	Keng Sang (20777263) (author), Changzheng Hong (21227694) (author), Zhihua Zhang (16756) (author), Changwei Liu (631801) (author), Wenyao Chen (1428964) (author), Chenxin Wu (5042900) (author), Yuxia Zhong (16431224) (author), Lina Li (292076) (author), Lei Hua (465535) (author), Xinggui Zhou (1428961) (author), De Chen (119865) (author), Weikang Yuan (1416418) (author), Xuezhi Duan (108966) (author)
Published:	2025
Subjects:	Biophysics Biochemistry Microbiology Pharmacology Biotechnology Evolutionary Biology Immunology Cancer Computational Biology Space Science Chemical Sciences not elsewhere classified Information Systems not elsewhere classified poor oxygen activation causes propylene overhydrogenation simultaneously enhanced activity selectivity remains challenging 2 </ sub traditional au catalysts high activity gold catalysts zeolite interfaces zeolite interface zeolite catalyst yet achieving state transition significantly promoting reduction dynamics pivotal generation phase separation magnitude enhancement janus configuration hydroperoxyl radicals hydrocarbons represents geometric promotions fence strategy epoxidation rates cup structure cornerstone reaction conventional gold chemical industry
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Assembling a Metastable Electron Fence within Gold-Zeolite Interfaces for Boosted Propylene Epoxidation

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