Fluorescent aminal linked porous organic polymer for reversible iodine capture and sensing

A novel triazene-anthracene-based fuorescent aminal linked porous organic polymer (TALPOP) was prepared via metal free-Schif base polycondensation reaction of 9,10-bis-(4,6-diamino-S-triazin2-yl)anthracene and 2-furaldehyde. The polymer has exceptional chemical and thermal stabilities and exhibit go...

وصف كامل

محفوظ في:
التفاصيل البيبلوغرافية
المؤلف الرئيسي: Sabri, Muhammad Ashraf (author)
مؤلفون آخرون: Al-Sayah, Mohammad (author), Sen, Susan (author), Ibrahim, Taleb (author), El-Kadri, Oussama (author)
التنسيق: article
منشور في: 2020
الموضوعات:
الوصول للمادة أونلاين:http://hdl.handle.net/11073/19797
الوسوم: إضافة وسم
لا توجد وسوم, كن أول من يضع وسما على هذه التسجيلة!
_version_ 1864513443679174656
author Sabri, Muhammad Ashraf
author2 Al-Sayah, Mohammad
Sen, Susan
Ibrahim, Taleb
El-Kadri, Oussama
author2_role author
author
author
author
author_facet Sabri, Muhammad Ashraf
Al-Sayah, Mohammad
Sen, Susan
Ibrahim, Taleb
El-Kadri, Oussama
author_role author
dc.creator.none.fl_str_mv Sabri, Muhammad Ashraf
Al-Sayah, Mohammad
Sen, Susan
Ibrahim, Taleb
El-Kadri, Oussama
dc.date.none.fl_str_mv 2020-10-01T10:58:37Z
2020-10-01T10:58:37Z
2020
dc.format.none.fl_str_mv application/pdf
dc.identifier.none.fl_str_mv Sabri, M.A., Al-Sayah, M.H., Sen, S. et al. Fluorescent aminal linked porous organic polymer for reversible iodine capture and sensing. Sci Rep 10, 15943 (2020). https://doi.org/10.1038/s41598-020-72697-x
2045-2322
http://hdl.handle.net/11073/19797
10.1038/s41598-020-72697-x
dc.language.none.fl_str_mv en_US
dc.publisher.none.fl_str_mv Nature
dc.relation.none.fl_str_mv https://doi.org/10.1038/s41598-020-72697-x
dc.subject.none.fl_str_mv Environmental impact
Materials science
Polymer chemistry
dc.title.none.fl_str_mv Fluorescent aminal linked porous organic polymer for reversible iodine capture and sensing
dc.type.none.fl_str_mv Peer-Reviewed
Published version
info:eu-repo/semantics/publishedVersion
info:eu-repo/semantics/article
description A novel triazene-anthracene-based fuorescent aminal linked porous organic polymer (TALPOP) was prepared via metal free-Schif base polycondensation reaction of 9,10-bis-(4,6-diamino-S-triazin2-yl)anthracene and 2-furaldehyde. The polymer has exceptional chemical and thermal stabilities and exhibit good porosity with Brunauer–Emmett–Teller surface area of 401 m2 g−1. The combination of such porosity along with the highly conjugated heteroatom-rich framework enabled the polymer to exhibit exceptional iodine vapor uptake of up to 314 wt % and reversible iodine adsorption in solution. Because of the inclusion of the anthracene moieties, the TALPOP exhibited excellent detection sensitivity towards iodine via forescence quenching with Ksv value of 2.9 × 103 L mol−1. The cost effective TALPOP along with its high uptake and sensing of iodine, make it an ideal material for environmental remediation.
format article
id aus_679f34991a28ff9760835f69a3d05b78
identifier_str_mv Sabri, M.A., Al-Sayah, M.H., Sen, S. et al. Fluorescent aminal linked porous organic polymer for reversible iodine capture and sensing. Sci Rep 10, 15943 (2020). https://doi.org/10.1038/s41598-020-72697-x
2045-2322
10.1038/s41598-020-72697-x
language_invalid_str_mv en_US
network_acronym_str aus
network_name_str aus
oai_identifier_str oai:repository.aus.edu:11073/19797
publishDate 2020
publisher.none.fl_str_mv Nature
repository.mail.fl_str_mv
repository.name.fl_str_mv
repository_id_str
spelling Fluorescent aminal linked porous organic polymer for reversible iodine capture and sensingSabri, Muhammad AshrafAl-Sayah, MohammadSen, SusanIbrahim, TalebEl-Kadri, OussamaEnvironmental impactMaterials sciencePolymer chemistryA novel triazene-anthracene-based fuorescent aminal linked porous organic polymer (TALPOP) was prepared via metal free-Schif base polycondensation reaction of 9,10-bis-(4,6-diamino-S-triazin2-yl)anthracene and 2-furaldehyde. The polymer has exceptional chemical and thermal stabilities and exhibit good porosity with Brunauer–Emmett–Teller surface area of 401 m2 g−1. The combination of such porosity along with the highly conjugated heteroatom-rich framework enabled the polymer to exhibit exceptional iodine vapor uptake of up to 314 wt % and reversible iodine adsorption in solution. Because of the inclusion of the anthracene moieties, the TALPOP exhibited excellent detection sensitivity towards iodine via forescence quenching with Ksv value of 2.9 × 103 L mol−1. The cost effective TALPOP along with its high uptake and sensing of iodine, make it an ideal material for environmental remediation.Nature2020-10-01T10:58:37Z2020-10-01T10:58:37Z2020Peer-ReviewedPublished versioninfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleapplication/pdfSabri, M.A., Al-Sayah, M.H., Sen, S. et al. Fluorescent aminal linked porous organic polymer for reversible iodine capture and sensing. Sci Rep 10, 15943 (2020). https://doi.org/10.1038/s41598-020-72697-x2045-2322http://hdl.handle.net/11073/1979710.1038/s41598-020-72697-xen_UShttps://doi.org/10.1038/s41598-020-72697-xoai:repository.aus.edu:11073/197972024-08-22T12:05:58Z
spellingShingle Fluorescent aminal linked porous organic polymer for reversible iodine capture and sensing
Sabri, Muhammad Ashraf
Environmental impact
Materials science
Polymer chemistry
status_str publishedVersion
title Fluorescent aminal linked porous organic polymer for reversible iodine capture and sensing
title_full Fluorescent aminal linked porous organic polymer for reversible iodine capture and sensing
title_fullStr Fluorescent aminal linked porous organic polymer for reversible iodine capture and sensing
title_full_unstemmed Fluorescent aminal linked porous organic polymer for reversible iodine capture and sensing
title_short Fluorescent aminal linked porous organic polymer for reversible iodine capture and sensing
title_sort Fluorescent aminal linked porous organic polymer for reversible iodine capture and sensing
topic Environmental impact
Materials science
Polymer chemistry
url http://hdl.handle.net/11073/19797