HBN Nanoparticle-Assisted Rapid Thermal Cycling for the Detection of Acanthamoeba

Acanthamoeba are widely distributed in the environment and are known to cause blinding keratitis and brain infections with greater than 90% mortality rate. Currently, polymerase chain reaction (PCR) is a highly sensitive and promising technique in Acanthamoeba detection. Remarkably, the rate of heat...

وصف كامل

محفوظ في:
التفاصيل البيبلوغرافية
المؤلف الرئيسي: Rasheed, Abdul Khaliq (author)
مؤلفون آخرون: Siddiqui, Ruqaiyyah (author), Ahmed, Salma Mohammed Kabir (author), Gabriel, Shobana (author), Jalal, Mohammed Zayan (author), John, Akbar (author), Khan, Naveed (author)
التنسيق: article
منشور في: 2020
الموضوعات:
الوصول للمادة أونلاين:http://hdl.handle.net/11073/21429
الوسوم: إضافة وسم
لا توجد وسوم, كن أول من يضع وسما على هذه التسجيلة!
_version_ 1864513431930929152
author Rasheed, Abdul Khaliq
author2 Siddiqui, Ruqaiyyah
Ahmed, Salma Mohammed Kabir
Gabriel, Shobana
Jalal, Mohammed Zayan
John, Akbar
Khan, Naveed
author2_role author
author
author
author
author
author
author_facet Rasheed, Abdul Khaliq
Siddiqui, Ruqaiyyah
Ahmed, Salma Mohammed Kabir
Gabriel, Shobana
Jalal, Mohammed Zayan
John, Akbar
Khan, Naveed
author_role author
dc.creator.none.fl_str_mv Rasheed, Abdul Khaliq
Siddiqui, Ruqaiyyah
Ahmed, Salma Mohammed Kabir
Gabriel, Shobana
Jalal, Mohammed Zayan
John, Akbar
Khan, Naveed
dc.date.none.fl_str_mv 2020
2021-04-20T10:02:31Z
2021-04-20T10:02:31Z
dc.format.none.fl_str_mv application/pdf
dc.identifier.none.fl_str_mv Rasheed, A.K.; Siddiqui, R.; Ahmed, S.M.K.; Gabriel, S.; Jalal, M.Z.; John, A.; Khan, N.A. hBN Nanoparticle-Assisted Rapid Thermal Cycling for the Detection of Acanthamoeba. Pathogens 2020, 9, 824. https://doi.org/10.3390/pathogens9100824
2076-0817
http://hdl.handle.net/11073/21429
10.3390/pathogens9100824
dc.language.none.fl_str_mv en_US
dc.publisher.none.fl_str_mv MDPI
dc.relation.none.fl_str_mv https://doi.org/10.3390/pathogens9100824
dc.subject.none.fl_str_mv NanoPCR
Hexagonal boron nitride
Thermal conductivity
Acanthamoeba
Pathogen
Bio-heat transfer
dc.title.none.fl_str_mv HBN Nanoparticle-Assisted Rapid Thermal Cycling for the Detection of Acanthamoeba
dc.type.none.fl_str_mv Peer-Reviewed
Published version
info:eu-repo/semantics/publishedVersion
info:eu-repo/semantics/article
description Acanthamoeba are widely distributed in the environment and are known to cause blinding keratitis and brain infections with greater than 90% mortality rate. Currently, polymerase chain reaction (PCR) is a highly sensitive and promising technique in Acanthamoeba detection. Remarkably, the rate of heating–cooling and convective heat transfer of the PCR tube is limited by low thermal conductivity of the reagents mixture. The addition of nanoparticles to the reaction has been an interesting approach that could augment the thermal conductivity of the mixture and subsequently enhance heat transfer through the PCR tube. Here, we have developed hexagonal boron nitride (hBN) nanoparticle-based PCR assay for the rapid detection of Acanthamoeba to amplify DNA from low amoeba cell density. As low as 1 X 10¯⁴ wt % was determined as the optimum concentration of hBN nanoparticles, which increased Acanthamoeba DNA yield up to ~16%. Further, it was able to reduce PCR temperature that led to a ~2.0-fold increase in Acanthamoeba DNA yield at an improved PCR specificity at 46.2 °C low annealing temperature. hBN nanoparticles further reduced standard PCR step time by 10 min and cycles by eight; thus, enhancing Acanthamoeba detection rapidly. Enhancement of Acanthamoeba PCR DNA yield is possibly due to the high adsorption affnity of hBN nanoparticles to purine (Guanine—G) due to the higher thermal conductivity achieved in the PCR mixture due to the addition of hBN. Although further research is needed to demonstrate these findings in clinical application, we propose that the interfacial layers, Brownian motion, and percolation network contribute to the enhanced thermal conductivity effect.
format article
id aus_9edddf0e13ef25ec8673d448e5888504
identifier_str_mv Rasheed, A.K.; Siddiqui, R.; Ahmed, S.M.K.; Gabriel, S.; Jalal, M.Z.; John, A.; Khan, N.A. hBN Nanoparticle-Assisted Rapid Thermal Cycling for the Detection of Acanthamoeba. Pathogens 2020, 9, 824. https://doi.org/10.3390/pathogens9100824
2076-0817
10.3390/pathogens9100824
language_invalid_str_mv en_US
network_acronym_str aus
network_name_str aus
oai_identifier_str oai:repository.aus.edu:11073/21429
publishDate 2020
publisher.none.fl_str_mv MDPI
repository.mail.fl_str_mv
repository.name.fl_str_mv
repository_id_str
spelling HBN Nanoparticle-Assisted Rapid Thermal Cycling for the Detection of AcanthamoebaRasheed, Abdul KhaliqSiddiqui, RuqaiyyahAhmed, Salma Mohammed KabirGabriel, ShobanaJalal, Mohammed ZayanJohn, AkbarKhan, NaveedNanoPCRHexagonal boron nitrideThermal conductivityAcanthamoebaPathogenBio-heat transferAcanthamoeba are widely distributed in the environment and are known to cause blinding keratitis and brain infections with greater than 90% mortality rate. Currently, polymerase chain reaction (PCR) is a highly sensitive and promising technique in Acanthamoeba detection. Remarkably, the rate of heating–cooling and convective heat transfer of the PCR tube is limited by low thermal conductivity of the reagents mixture. The addition of nanoparticles to the reaction has been an interesting approach that could augment the thermal conductivity of the mixture and subsequently enhance heat transfer through the PCR tube. Here, we have developed hexagonal boron nitride (hBN) nanoparticle-based PCR assay for the rapid detection of Acanthamoeba to amplify DNA from low amoeba cell density. As low as 1 X 10¯⁴ wt % was determined as the optimum concentration of hBN nanoparticles, which increased Acanthamoeba DNA yield up to ~16%. Further, it was able to reduce PCR temperature that led to a ~2.0-fold increase in Acanthamoeba DNA yield at an improved PCR specificity at 46.2 °C low annealing temperature. hBN nanoparticles further reduced standard PCR step time by 10 min and cycles by eight; thus, enhancing Acanthamoeba detection rapidly. Enhancement of Acanthamoeba PCR DNA yield is possibly due to the high adsorption affnity of hBN nanoparticles to purine (Guanine—G) due to the higher thermal conductivity achieved in the PCR mixture due to the addition of hBN. Although further research is needed to demonstrate these findings in clinical application, we propose that the interfacial layers, Brownian motion, and percolation network contribute to the enhanced thermal conductivity effect.American University of SharjahMDPI2021-04-20T10:02:31Z2021-04-20T10:02:31Z2020Peer-ReviewedPublished versioninfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleapplication/pdfRasheed, A.K.; Siddiqui, R.; Ahmed, S.M.K.; Gabriel, S.; Jalal, M.Z.; John, A.; Khan, N.A. hBN Nanoparticle-Assisted Rapid Thermal Cycling for the Detection of Acanthamoeba. Pathogens 2020, 9, 824. https://doi.org/10.3390/pathogens91008242076-0817http://hdl.handle.net/11073/2142910.3390/pathogens9100824en_UShttps://doi.org/10.3390/pathogens9100824oai:repository.aus.edu:11073/214292024-08-22T11:59:40Z
spellingShingle HBN Nanoparticle-Assisted Rapid Thermal Cycling for the Detection of Acanthamoeba
Rasheed, Abdul Khaliq
NanoPCR
Hexagonal boron nitride
Thermal conductivity
Acanthamoeba
Pathogen
Bio-heat transfer
status_str publishedVersion
title HBN Nanoparticle-Assisted Rapid Thermal Cycling for the Detection of Acanthamoeba
title_full HBN Nanoparticle-Assisted Rapid Thermal Cycling for the Detection of Acanthamoeba
title_fullStr HBN Nanoparticle-Assisted Rapid Thermal Cycling for the Detection of Acanthamoeba
title_full_unstemmed HBN Nanoparticle-Assisted Rapid Thermal Cycling for the Detection of Acanthamoeba
title_short HBN Nanoparticle-Assisted Rapid Thermal Cycling for the Detection of Acanthamoeba
title_sort HBN Nanoparticle-Assisted Rapid Thermal Cycling for the Detection of Acanthamoeba
topic NanoPCR
Hexagonal boron nitride
Thermal conductivity
Acanthamoeba
Pathogen
Bio-heat transfer
url http://hdl.handle.net/11073/21429