Tailoring Cu immobilized MCM-41-based mesostructured catalysts for selective hydrogenolysis of biomass-derived furfural

The CuO-supported MCM-41 catalysts were prepared using a simple incipient wet impregnation method. The catalysts were investigated for hydrogenation of furfural to furfuryl alcohol synthesis. Among all the catalysts, the 2.5% CuO/MCM-41 catalyst shows the best catalytic performance with 92.5% conver...

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Main Author: Leela Prasad, Yandrati (author)
Other Authors: Sekhar Kaladi, Swamy (author), Gundeboyina, Raveendra (author), Pothu, Ramakrishna (author), Moli, Vijaya (author), Venkateswara Rao, B. (author), Boddula, Rajender (author), Devulapalli, Rammohanrao (author), Mitta, Harisekhar (author)
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Published: 2024
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Online Access:http://dx.doi.org/10.1016/j.catcom.2024.106898
https://www.sciencedirect.com/science/article/pii/S156673672400058X
http://hdl.handle.net/10576/65064
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author Leela Prasad, Yandrati
author2 Sekhar Kaladi, Swamy
Gundeboyina, Raveendra
Pothu, Ramakrishna
Moli, Vijaya
Venkateswara Rao, B.
Boddula, Rajender
Devulapalli, Rammohanrao
Mitta, Harisekhar
author2_role author
author
author
author
author
author
author
author
author_facet Leela Prasad, Yandrati
Sekhar Kaladi, Swamy
Gundeboyina, Raveendra
Pothu, Ramakrishna
Moli, Vijaya
Venkateswara Rao, B.
Boddula, Rajender
Devulapalli, Rammohanrao
Mitta, Harisekhar
author_role author
dc.creator.none.fl_str_mv Leela Prasad, Yandrati
Sekhar Kaladi, Swamy
Gundeboyina, Raveendra
Pothu, Ramakrishna
Moli, Vijaya
Venkateswara Rao, B.
Boddula, Rajender
Devulapalli, Rammohanrao
Mitta, Harisekhar
dc.date.none.fl_str_mv 2024-02-29
2025-05-20T08:06:34Z
dc.format.none.fl_str_mv application/pdf
dc.identifier.none.fl_str_mv http://dx.doi.org/10.1016/j.catcom.2024.106898
15667367
https://www.sciencedirect.com/science/article/pii/S156673672400058X
http://hdl.handle.net/10576/65064
187
dc.language.none.fl_str_mv en
dc.publisher.none.fl_str_mv Elsevier
dc.rights.none.fl_str_mv http://creativecommons.org/licenses/by-nc-nd/4.0/
info:eu-repo/semantics/openAccess
dc.subject.none.fl_str_mv Hydrogenation
Furfural
Furfuryl alcohol
CuO
MCM-41
Sustainability energy & fuels
Green chemistry
dc.title.none.fl_str_mv Tailoring Cu immobilized MCM-41-based mesostructured catalysts for selective hydrogenolysis of biomass-derived furfural
dc.type.none.fl_str_mv Article
info:eu-repo/semantics/publishedVersion
info:eu-repo/semantics/article
description The CuO-supported MCM-41 catalysts were prepared using a simple incipient wet impregnation method. The catalysts were investigated for hydrogenation of furfural to furfuryl alcohol synthesis. Among all the catalysts, the 2.5% CuO/MCM-41 catalyst shows the best catalytic performance with 92.5% conversion and 89% selectivity of furfuryl alcohol at 210 °C. The catalyst also demonstrated a high turnover frequency (TOF) of 154.4 h−1. The 2.5% CuO/MCM-41 catalyst remained stable for up to 20 h during the time on stream.
eu_rights_str_mv openAccess
format article
id qu_2ad9b995a67f181374e278e716853114
identifier_str_mv 15667367
187
language_invalid_str_mv en
network_acronym_str qu
network_name_str Qatar University repository
oai_identifier_str oai:qspace.qu.edu.qa:10576/65064
publishDate 2024
publisher.none.fl_str_mv Elsevier
repository.mail.fl_str_mv
repository.name.fl_str_mv
repository_id_str
rights_invalid_str_mv http://creativecommons.org/licenses/by-nc-nd/4.0/
spelling Tailoring Cu immobilized MCM-41-based mesostructured catalysts for selective hydrogenolysis of biomass-derived furfuralLeela Prasad, YandratiSekhar Kaladi, SwamyGundeboyina, RaveendraPothu, RamakrishnaMoli, VijayaVenkateswara Rao, B.Boddula, RajenderDevulapalli, RammohanraoMitta, HarisekharHydrogenationFurfuralFurfuryl alcoholCuOMCM-41Sustainability energy & fuelsGreen chemistryThe CuO-supported MCM-41 catalysts were prepared using a simple incipient wet impregnation method. The catalysts were investigated for hydrogenation of furfural to furfuryl alcohol synthesis. Among all the catalysts, the 2.5% CuO/MCM-41 catalyst shows the best catalytic performance with 92.5% conversion and 89% selectivity of furfuryl alcohol at 210 °C. The catalyst also demonstrated a high turnover frequency (TOF) of 154.4 h−1. The 2.5% CuO/MCM-41 catalyst remained stable for up to 20 h during the time on stream.Elsevier2025-05-20T08:06:34Z2024-02-29Articleinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleapplication/pdfhttp://dx.doi.org/10.1016/j.catcom.2024.10689815667367https://www.sciencedirect.com/science/article/pii/S156673672400058Xhttp://hdl.handle.net/10576/65064187enhttp://creativecommons.org/licenses/by-nc-nd/4.0/info:eu-repo/semantics/openAccessoai:qspace.qu.edu.qa:10576/650642025-05-20T19:08:31Z
spellingShingle Tailoring Cu immobilized MCM-41-based mesostructured catalysts for selective hydrogenolysis of biomass-derived furfural
Leela Prasad, Yandrati
Hydrogenation
Furfural
Furfuryl alcohol
CuO
MCM-41
Sustainability energy & fuels
Green chemistry
status_str publishedVersion
title Tailoring Cu immobilized MCM-41-based mesostructured catalysts for selective hydrogenolysis of biomass-derived furfural
title_full Tailoring Cu immobilized MCM-41-based mesostructured catalysts for selective hydrogenolysis of biomass-derived furfural
title_fullStr Tailoring Cu immobilized MCM-41-based mesostructured catalysts for selective hydrogenolysis of biomass-derived furfural
title_full_unstemmed Tailoring Cu immobilized MCM-41-based mesostructured catalysts for selective hydrogenolysis of biomass-derived furfural
title_short Tailoring Cu immobilized MCM-41-based mesostructured catalysts for selective hydrogenolysis of biomass-derived furfural
title_sort Tailoring Cu immobilized MCM-41-based mesostructured catalysts for selective hydrogenolysis of biomass-derived furfural
topic Hydrogenation
Furfural
Furfuryl alcohol
CuO
MCM-41
Sustainability energy & fuels
Green chemistry
url http://dx.doi.org/10.1016/j.catcom.2024.106898
https://www.sciencedirect.com/science/article/pii/S156673672400058X
http://hdl.handle.net/10576/65064