Natural resorcylic acid lactones: A chemical biology approach for anticancer activity

Resorcylic acid lactones (RALs) are fungal polyketides that consist of a β-resorcylic acid residue (2,4-dihydroxybenzoic acid) embedded in a macrolactone ring. RALs exhibit a broad range of biological activities, including anticancer activities. Following discovery of the selective Hsp90 inhibition...

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محفوظ في:
التفاصيل البيبلوغرافية
المؤلف الرئيسي: Shilpa, Kuttikrishnan (author)
مؤلفون آخرون: Prabhu, Kirti S. (author), Al Sharie, Ahmed H. (author), Al Zu'bi, Yazan O. (author), Alali, Feras Q. (author), Oberlies, Nicholas H. (author), Ahmad, Aamir (author), El-Elimat, Tamam (author), Uddin, Shahab (author)
التنسيق: article
منشور في: 2022
الموضوعات:
الوصول للمادة أونلاين:http://dx.doi.org/10.1016/j.drudis.2021.10.001
https://www.sciencedirect.com/science/article/pii/S1359644621004323
http://hdl.handle.net/10576/41837
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author Shilpa, Kuttikrishnan
author2 Prabhu, Kirti S.
Al Sharie, Ahmed H.
Al Zu'bi, Yazan O.
Alali, Feras Q.
Oberlies, Nicholas H.
Ahmad, Aamir
El-Elimat, Tamam
Uddin, Shahab
author2_role author
author
author
author
author
author
author
author
author_facet Shilpa, Kuttikrishnan
Prabhu, Kirti S.
Al Sharie, Ahmed H.
Al Zu'bi, Yazan O.
Alali, Feras Q.
Oberlies, Nicholas H.
Ahmad, Aamir
El-Elimat, Tamam
Uddin, Shahab
author_role author
dc.creator.none.fl_str_mv Shilpa, Kuttikrishnan
Prabhu, Kirti S.
Al Sharie, Ahmed H.
Al Zu'bi, Yazan O.
Alali, Feras Q.
Oberlies, Nicholas H.
Ahmad, Aamir
El-Elimat, Tamam
Uddin, Shahab
dc.date.none.fl_str_mv 2022-02-28
2023-04-12T05:34:39Z
dc.format.none.fl_str_mv application/pdf
dc.identifier.none.fl_str_mv http://dx.doi.org/10.1016/j.drudis.2021.10.001
Kuttikrishnan, Shilpa, Kirti S. Prabhu, Ahmed H. Al Sharie, Yazan O. Al Zu'bi, Feras Q. Alali, Nicholas H. Oberlies, Aamir Ahmad, Tamam El-Elimat, and Shahab Uddin. "Natural resorcylic acid lactones: A chemical biology approach for anticancer activity." Drug Discovery Today 27, no. 2 (2022): 547-557.
13596446
https://www.sciencedirect.com/science/article/pii/S1359644621004323
http://hdl.handle.net/10576/41837
547-557
2
27
dc.language.none.fl_str_mv en
dc.publisher.none.fl_str_mv Elsevier
dc.rights.none.fl_str_mv http://creativecommons.org/licenses/by/4.0/
info:eu-repo/semantics/openAccess
dc.subject.none.fl_str_mv Resorcylic acid lactones
Heat shock protein 90 inhibitors
Protein kinase inhibitors
Radicicol
Hypothemycin
5Z-7-oxo-zeaenol
dc.title.none.fl_str_mv Natural resorcylic acid lactones: A chemical biology approach for anticancer activity
dc.type.none.fl_str_mv Article
info:eu-repo/semantics/publishedVersion
info:eu-repo/semantics/article
description Resorcylic acid lactones (RALs) are fungal polyketides that consist of a β-resorcylic acid residue (2,4-dihydroxybenzoic acid) embedded in a macrolactone ring. RALs exhibit a broad range of biological activities, including anticancer activities. Following discovery of the selective Hsp90 inhibition activity of radicicol, the kinase inhibition activity of hypothemycin, monocillin II, 5Z-7-oxo-zeaenol, and L-783,277 RALs, and the nuclear factor kappa B (NF-κB) inhibition activity of the RAL zearalenone, have attracted great attention as potential therapeutics for cancer treatment. In this minireview, we focus on natural RALs that possess cytotoxic activities [IC50 values < 10 μM (or 4–5 μg/ml)], discussing their structures, isolation, occurrence, biological activities, and anticancer molecular mechanisms.
eu_rights_str_mv openAccess
format article
id qu_69481247cbdbc58a52639b605930d260
identifier_str_mv Kuttikrishnan, Shilpa, Kirti S. Prabhu, Ahmed H. Al Sharie, Yazan O. Al Zu'bi, Feras Q. Alali, Nicholas H. Oberlies, Aamir Ahmad, Tamam El-Elimat, and Shahab Uddin. "Natural resorcylic acid lactones: A chemical biology approach for anticancer activity." Drug Discovery Today 27, no. 2 (2022): 547-557.
13596446
547-557
2
27
language_invalid_str_mv en
network_acronym_str qu
network_name_str Qatar University repository
oai_identifier_str oai:qspace.qu.edu.qa:10576/41837
publishDate 2022
publisher.none.fl_str_mv Elsevier
repository.mail.fl_str_mv
repository.name.fl_str_mv
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rights_invalid_str_mv http://creativecommons.org/licenses/by/4.0/
spelling Natural resorcylic acid lactones: A chemical biology approach for anticancer activityShilpa, KuttikrishnanPrabhu, Kirti S.Al Sharie, Ahmed H.Al Zu'bi, Yazan O.Alali, Feras Q.Oberlies, Nicholas H.Ahmad, AamirEl-Elimat, TamamUddin, ShahabResorcylic acid lactonesHeat shock protein 90 inhibitorsProtein kinase inhibitorsRadicicolHypothemycin5Z-7-oxo-zeaenolResorcylic acid lactones (RALs) are fungal polyketides that consist of a β-resorcylic acid residue (2,4-dihydroxybenzoic acid) embedded in a macrolactone ring. RALs exhibit a broad range of biological activities, including anticancer activities. Following discovery of the selective Hsp90 inhibition activity of radicicol, the kinase inhibition activity of hypothemycin, monocillin II, 5Z-7-oxo-zeaenol, and L-783,277 RALs, and the nuclear factor kappa B (NF-κB) inhibition activity of the RAL zearalenone, have attracted great attention as potential therapeutics for cancer treatment. In this minireview, we focus on natural RALs that possess cytotoxic activities [IC50 values < 10 μM (or 4–5 μg/ml)], discussing their structures, isolation, occurrence, biological activities, and anticancer molecular mechanisms.This work is supported by funding from the Medical Research Center (grant no. MRC-01-21-301 (SU)), Hamad Medical Corporation, Doha, Qatar. The authors acknowledge Qatar National Library, Doha, Qatar for supporting Open Access funding for this article.Elsevier2023-04-12T05:34:39Z2022-02-28Articleinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleapplication/pdfhttp://dx.doi.org/10.1016/j.drudis.2021.10.001Kuttikrishnan, Shilpa, Kirti S. Prabhu, Ahmed H. Al Sharie, Yazan O. Al Zu'bi, Feras Q. Alali, Nicholas H. Oberlies, Aamir Ahmad, Tamam El-Elimat, and Shahab Uddin. "Natural resorcylic acid lactones: A chemical biology approach for anticancer activity." Drug Discovery Today 27, no. 2 (2022): 547-557.13596446https://www.sciencedirect.com/science/article/pii/S1359644621004323http://hdl.handle.net/10576/41837547-557227enhttp://creativecommons.org/licenses/by/4.0/info:eu-repo/semantics/openAccessoai:qspace.qu.edu.qa:10576/418372024-07-23T10:58:21Z
spellingShingle Natural resorcylic acid lactones: A chemical biology approach for anticancer activity
Shilpa, Kuttikrishnan
Resorcylic acid lactones
Heat shock protein 90 inhibitors
Protein kinase inhibitors
Radicicol
Hypothemycin
5Z-7-oxo-zeaenol
status_str publishedVersion
title Natural resorcylic acid lactones: A chemical biology approach for anticancer activity
title_full Natural resorcylic acid lactones: A chemical biology approach for anticancer activity
title_fullStr Natural resorcylic acid lactones: A chemical biology approach for anticancer activity
title_full_unstemmed Natural resorcylic acid lactones: A chemical biology approach for anticancer activity
title_short Natural resorcylic acid lactones: A chemical biology approach for anticancer activity
title_sort Natural resorcylic acid lactones: A chemical biology approach for anticancer activity
topic Resorcylic acid lactones
Heat shock protein 90 inhibitors
Protein kinase inhibitors
Radicicol
Hypothemycin
5Z-7-oxo-zeaenol
url http://dx.doi.org/10.1016/j.drudis.2021.10.001
https://www.sciencedirect.com/science/article/pii/S1359644621004323
http://hdl.handle.net/10576/41837