Design and optimization of four-terminal mechanically stacked and optically coupled silicon/perovskite tandem solar cells with over 28% efficiency

Silicon/perovskite tandem devices are believed to be a favorite contender for improving cell performance over the theoretical maximum value of single-junction photovoltaic (PV) cells. The present study evaluates the design and optimization of four-terminal (4-T) mechanically stacked and optically co...

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Main Author: Ehsan, Raza (author)
Other Authors: Ahmad, Zubair (author), Aziz, Fakhra (author), Asif, Muhammad (author), Mehmood, Muhammad Qasim (author), Bhadra, Jolly (author), Al-Thani, Noora J. (author)
Format: article
Published: 2023
Subjects:
Online Access:http://dx.doi.org/10.1016/j.heliyon.2023.e13477
https://www.sciencedirect.com/science/article/pii/S2405844023006849
http://hdl.handle.net/10576/40354
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_version_ 1857415084531253248
author Ehsan, Raza
author2 Ahmad, Zubair
Aziz, Fakhra
Asif, Muhammad
Mehmood, Muhammad Qasim
Bhadra, Jolly
Al-Thani, Noora J.
author2_role author
author
author
author
author
author
author_facet Ehsan, Raza
Ahmad, Zubair
Aziz, Fakhra
Asif, Muhammad
Mehmood, Muhammad Qasim
Bhadra, Jolly
Al-Thani, Noora J.
author_role author
dc.creator.none.fl_str_mv Ehsan, Raza
Ahmad, Zubair
Aziz, Fakhra
Asif, Muhammad
Mehmood, Muhammad Qasim
Bhadra, Jolly
Al-Thani, Noora J.
dc.date.none.fl_str_mv 2023-02-26T06:56:55Z
2023
dc.format.none.fl_str_mv application/pdf
dc.identifier.none.fl_str_mv http://dx.doi.org/10.1016/j.heliyon.2023.e13477
Raza E, Ahmad Z, Aziz F, Asif M, Mehmood MQ, Bhadra J, Al-Thani NJ. Design and optimization of four-terminal mechanically stacked and optically coupled silicon/perovskite tandem solar cells with over 28% efficiency. Heliyon. 2023 Feb 3;9(2):e13477. doi: 10.1016/j.heliyon.2023.e13477.
24058440
https://www.sciencedirect.com/science/article/pii/S2405844023006849
http://hdl.handle.net/10576/40354
2
9
dc.language.none.fl_str_mv en
dc.publisher.none.fl_str_mv Elsevier
dc.rights.none.fl_str_mv http://creativecommons.org/licenses/by/4.0/
info:eu-repo/semantics/openAccess
dc.subject.none.fl_str_mv HTM-Free perovskite PV cells
Crystalline silicon solar cells
Mechanically stacked four-terminal tandem
Optically coupled four-terminal tandem
SCAPS-1D
Energy conversion efficiency
dc.title.none.fl_str_mv Design and optimization of four-terminal mechanically stacked and optically coupled silicon/perovskite tandem solar cells with over 28% efficiency
dc.type.none.fl_str_mv Article
info:eu-repo/semantics/publishedVersion
info:eu-repo/semantics/article
description Silicon/perovskite tandem devices are believed to be a favorite contender for improving cell performance over the theoretical maximum value of single-junction photovoltaic (PV) cells. The present study evaluates the design and optimization of four-terminal (4-T) mechanically stacked and optically coupled configurations using SCAPS (solar cell capacitance simulator). Low-cost, stable, and easily processed semitransparent carbon electrode-based perovskite solar cells (c-PSCs) without hole transport material (HTM) and highly efficient crystalline silicon (c-Si) PV cells were utilized as top and bottom cells, respectively. The wide bandgap multi-cation perovskite Csx(FA0.4MA0.6)1−xPbI2.8Br0.2 and a low bandgap c-Si were employed as light-harvesting layers in the top and bottom cells, respectively. The impact of perovskite thickness and doping concentrations were examined and optimized for both tandem configurations. Under optimized conditions, thicknesses of 1000 nm and 1100 nm are the best values of the perovskite absorber layer for 4-T mechanically stacked and optically coupled arrangements, respectively. Likewise, 1 × 1017 cm−3 doping concentration of top cells revealed the highest performance in both structures. With these optimized parameters under tandem configurations, efficiency values of 28.38% and 29.34% were obtained in 4-T mechanically and optically coupled tandems, respectively. Results suggest that by optimizing perovskite thickness and doping concentration, the proposed designs using HTM-free c-PSCs could enhance device performance.
eu_rights_str_mv openAccess
format article
id qu_8b938733d1b4b4979886ea321e8e8526
identifier_str_mv Raza E, Ahmad Z, Aziz F, Asif M, Mehmood MQ, Bhadra J, Al-Thani NJ. Design and optimization of four-terminal mechanically stacked and optically coupled silicon/perovskite tandem solar cells with over 28% efficiency. Heliyon. 2023 Feb 3;9(2):e13477. doi: 10.1016/j.heliyon.2023.e13477.
24058440
2
9
language_invalid_str_mv en
network_acronym_str qu
network_name_str Qatar University repository
oai_identifier_str oai:qspace.qu.edu.qa:10576/40354
publishDate 2023
publisher.none.fl_str_mv Elsevier
repository.mail.fl_str_mv
repository.name.fl_str_mv
repository_id_str
rights_invalid_str_mv http://creativecommons.org/licenses/by/4.0/
spelling Design and optimization of four-terminal mechanically stacked and optically coupled silicon/perovskite tandem solar cells with over 28% efficiencyEhsan, RazaAhmad, ZubairAziz, FakhraAsif, MuhammadMehmood, Muhammad QasimBhadra, JollyAl-Thani, Noora J.HTM-Free perovskite PV cellsCrystalline silicon solar cellsMechanically stacked four-terminal tandemOptically coupled four-terminal tandemSCAPS-1DEnergy conversion efficiencySilicon/perovskite tandem devices are believed to be a favorite contender for improving cell performance over the theoretical maximum value of single-junction photovoltaic (PV) cells. The present study evaluates the design and optimization of four-terminal (4-T) mechanically stacked and optically coupled configurations using SCAPS (solar cell capacitance simulator). Low-cost, stable, and easily processed semitransparent carbon electrode-based perovskite solar cells (c-PSCs) without hole transport material (HTM) and highly efficient crystalline silicon (c-Si) PV cells were utilized as top and bottom cells, respectively. The wide bandgap multi-cation perovskite Csx(FA0.4MA0.6)1−xPbI2.8Br0.2 and a low bandgap c-Si were employed as light-harvesting layers in the top and bottom cells, respectively. The impact of perovskite thickness and doping concentrations were examined and optimized for both tandem configurations. Under optimized conditions, thicknesses of 1000 nm and 1100 nm are the best values of the perovskite absorber layer for 4-T mechanically stacked and optically coupled arrangements, respectively. Likewise, 1 × 1017 cm−3 doping concentration of top cells revealed the highest performance in both structures. With these optimized parameters under tandem configurations, efficiency values of 28.38% and 29.34% were obtained in 4-T mechanically and optically coupled tandems, respectively. Results suggest that by optimizing perovskite thickness and doping concentration, the proposed designs using HTM-free c-PSCs could enhance device performance.The article processing charges (APCs) are funded by the Qatar National Library, Qatar.Elsevier2023-02-26T06:56:55Z2023Articleinfo:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/articleapplication/pdfhttp://dx.doi.org/10.1016/j.heliyon.2023.e13477Raza E, Ahmad Z, Aziz F, Asif M, Mehmood MQ, Bhadra J, Al-Thani NJ. Design and optimization of four-terminal mechanically stacked and optically coupled silicon/perovskite tandem solar cells with over 28% efficiency. Heliyon. 2023 Feb 3;9(2):e13477. doi: 10.1016/j.heliyon.2023.e13477.24058440https://www.sciencedirect.com/science/article/pii/S2405844023006849http://hdl.handle.net/10576/4035429enhttp://creativecommons.org/licenses/by/4.0/info:eu-repo/semantics/openAccessoai:qspace.qu.edu.qa:10576/403542024-07-23T13:52:35Z
spellingShingle Design and optimization of four-terminal mechanically stacked and optically coupled silicon/perovskite tandem solar cells with over 28% efficiency
Ehsan, Raza
HTM-Free perovskite PV cells
Crystalline silicon solar cells
Mechanically stacked four-terminal tandem
Optically coupled four-terminal tandem
SCAPS-1D
Energy conversion efficiency
status_str publishedVersion
title Design and optimization of four-terminal mechanically stacked and optically coupled silicon/perovskite tandem solar cells with over 28% efficiency
title_full Design and optimization of four-terminal mechanically stacked and optically coupled silicon/perovskite tandem solar cells with over 28% efficiency
title_fullStr Design and optimization of four-terminal mechanically stacked and optically coupled silicon/perovskite tandem solar cells with over 28% efficiency
title_full_unstemmed Design and optimization of four-terminal mechanically stacked and optically coupled silicon/perovskite tandem solar cells with over 28% efficiency
title_short Design and optimization of four-terminal mechanically stacked and optically coupled silicon/perovskite tandem solar cells with over 28% efficiency
title_sort Design and optimization of four-terminal mechanically stacked and optically coupled silicon/perovskite tandem solar cells with over 28% efficiency
topic HTM-Free perovskite PV cells
Crystalline silicon solar cells
Mechanically stacked four-terminal tandem
Optically coupled four-terminal tandem
SCAPS-1D
Energy conversion efficiency
url http://dx.doi.org/10.1016/j.heliyon.2023.e13477
https://www.sciencedirect.com/science/article/pii/S2405844023006849
http://hdl.handle.net/10576/40354