Increased Crystal Field Drives Intermediate Coupling and Minimizes Decoherence in Tetravalent Praseodymium Qubits by Arun Ramanathan (9992643)

“…Herein, the magnitude of the CF is increased via control of the RE oxidation state. The enhanced 4f metal–ligand covalency in Pr⁴⁺ gives rise to CF energy scales that compete with the spin–orbit coupling of Pr⁴⁺ and thereby shifts the paradigm from the ionic ζ_SOC ≫ <i>V</i>_CF limit, used to describe trivalent RE-ion, to an intermediate coupling (IC) regime. …”

Increased Crystal Field Drives Intermediate Coupling and Minimizes Decoherence in Tetravalent Praseodymium Qubits by Arun Ramanathan (9992643)

“…Herein, the magnitude of the CF is increased via control of the RE oxidation state. The enhanced 4f metal–ligand covalency in Pr⁴⁺ gives rise to CF energy scales that compete with the spin–orbit coupling of Pr⁴⁺ and thereby shifts the paradigm from the ionic ζ_SOC ≫ <i>V</i>_CF limit, used to describe trivalent RE-ion, to an intermediate coupling (IC) regime. …”

Increased Crystal Field Drives Intermediate Coupling and Minimizes Decoherence in Tetravalent Praseodymium Qubits by Arun Ramanathan (9992643)

“…Herein, the magnitude of the CF is increased via control of the RE oxidation state. The enhanced 4f metal–ligand covalency in Pr⁴⁺ gives rise to CF energy scales that compete with the spin–orbit coupling of Pr⁴⁺ and thereby shifts the paradigm from the ionic ζ_SOC ≫ <i>V</i>_CF limit, used to describe trivalent RE-ion, to an intermediate coupling (IC) regime. …”

Increased Crystal Field Drives Intermediate Coupling and Minimizes Decoherence in Tetravalent Praseodymium Qubits by Arun Ramanathan (9992643)

“…Herein, the magnitude of the CF is increased via control of the RE oxidation state. The enhanced 4f metal–ligand covalency in Pr⁴⁺ gives rise to CF energy scales that compete with the spin–orbit coupling of Pr⁴⁺ and thereby shifts the paradigm from the ionic ζ_SOC ≫ <i>V</i>_CF limit, used to describe trivalent RE-ion, to an intermediate coupling (IC) regime. …”

Increased Crystal Field Drives Intermediate Coupling and Minimizes Decoherence in Tetravalent Praseodymium Qubits by Arun Ramanathan (9992643)

“…Herein, the magnitude of the CF is increased via control of the RE oxidation state. The enhanced 4f metal–ligand covalency in Pr⁴⁺ gives rise to CF energy scales that compete with the spin–orbit coupling of Pr⁴⁺ and thereby shifts the paradigm from the ionic ζ_SOC ≫ <i>V</i>_CF limit, used to describe trivalent RE-ion, to an intermediate coupling (IC) regime. …”

Increased Crystal Field Drives Intermediate Coupling and Minimizes Decoherence in Tetravalent Praseodymium Qubits by Arun Ramanathan (9992643)

“…Herein, the magnitude of the CF is increased via control of the RE oxidation state. The enhanced 4f metal–ligand covalency in Pr⁴⁺ gives rise to CF energy scales that compete with the spin–orbit coupling of Pr⁴⁺ and thereby shifts the paradigm from the ionic ζ_SOC ≫ <i>V</i>_CF limit, used to describe trivalent RE-ion, to an intermediate coupling (IC) regime. …”

Increased Crystal Field Drives Intermediate Coupling and Minimizes Decoherence in Tetravalent Praseodymium Qubits by Arun Ramanathan (9992643)

“…Herein, the magnitude of the CF is increased via control of the RE oxidation state. The enhanced 4f metal–ligand covalency in Pr⁴⁺ gives rise to CF energy scales that compete with the spin–orbit coupling of Pr⁴⁺ and thereby shifts the paradigm from the ionic ζ_SOC ≫ <i>V</i>_CF limit, used to describe trivalent RE-ion, to an intermediate coupling (IC) regime. …”

Increased Crystal Field Drives Intermediate Coupling and Minimizes Decoherence in Tetravalent Praseodymium Qubits by Arun Ramanathan (9992643)

“…Herein, the magnitude of the CF is increased via control of the RE oxidation state. The enhanced 4f metal–ligand covalency in Pr⁴⁺ gives rise to CF energy scales that compete with the spin–orbit coupling of Pr⁴⁺ and thereby shifts the paradigm from the ionic ζ_SOC ≫ <i>V</i>_CF limit, used to describe trivalent RE-ion, to an intermediate coupling (IC) regime. …”

Increased Crystal Field Drives Intermediate Coupling and Minimizes Decoherence in Tetravalent Praseodymium Qubits by Arun Ramanathan (9992643)

“…Herein, the magnitude of the CF is increased via control of the RE oxidation state. The enhanced 4f metal–ligand covalency in Pr⁴⁺ gives rise to CF energy scales that compete with the spin–orbit coupling of Pr⁴⁺ and thereby shifts the paradigm from the ionic ζ_SOC ≫ <i>V</i>_CF limit, used to describe trivalent RE-ion, to an intermediate coupling (IC) regime. …”

Increased Crystal Field Drives Intermediate Coupling and Minimizes Decoherence in Tetravalent Praseodymium Qubits by Arun Ramanathan (9992643)

“…Herein, the magnitude of the CF is increased via control of the RE oxidation state. The enhanced 4f metal–ligand covalency in Pr⁴⁺ gives rise to CF energy scales that compete with the spin–orbit coupling of Pr⁴⁺ and thereby shifts the paradigm from the ionic ζ_SOC ≫ <i>V</i>_CF limit, used to describe trivalent RE-ion, to an intermediate coupling (IC) regime. …”

Increased Crystal Field Drives Intermediate Coupling and Minimizes Decoherence in Tetravalent Praseodymium Qubits by Arun Ramanathan (9992643)

“…Herein, the magnitude of the CF is increased via control of the RE oxidation state. The enhanced 4f metal–ligand covalency in Pr⁴⁺ gives rise to CF energy scales that compete with the spin–orbit coupling of Pr⁴⁺ and thereby shifts the paradigm from the ionic ζ_SOC ≫ <i>V</i>_CF limit, used to describe trivalent RE-ion, to an intermediate coupling (IC) regime. …”

Increased Crystal Field Drives Intermediate Coupling and Minimizes Decoherence in Tetravalent Praseodymium Qubits by Arun Ramanathan (9992643)

“…Herein, the magnitude of the CF is increased via control of the RE oxidation state. The enhanced 4f metal–ligand covalency in Pr⁴⁺ gives rise to CF energy scales that compete with the spin–orbit coupling of Pr⁴⁺ and thereby shifts the paradigm from the ionic ζ_SOC ≫ <i>V</i>_CF limit, used to describe trivalent RE-ion, to an intermediate coupling (IC) regime. …”

Increased Crystal Field Drives Intermediate Coupling and Minimizes Decoherence in Tetravalent Praseodymium Qubits by Arun Ramanathan (9992643)

“…Herein, the magnitude of the CF is increased via control of the RE oxidation state. The enhanced 4f metal–ligand covalency in Pr⁴⁺ gives rise to CF energy scales that compete with the spin–orbit coupling of Pr⁴⁺ and thereby shifts the paradigm from the ionic ζ_SOC ≫ <i>V</i>_CF limit, used to describe trivalent RE-ion, to an intermediate coupling (IC) regime. …”

Increased Crystal Field Drives Intermediate Coupling and Minimizes Decoherence in Tetravalent Praseodymium Qubits by Arun Ramanathan (9992643)

“…Herein, the magnitude of the CF is increased via control of the RE oxidation state. The enhanced 4f metal–ligand covalency in Pr⁴⁺ gives rise to CF energy scales that compete with the spin–orbit coupling of Pr⁴⁺ and thereby shifts the paradigm from the ionic ζ_SOC ≫ <i>V</i>_CF limit, used to describe trivalent RE-ion, to an intermediate coupling (IC) regime. …”

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