Nuclear Quantum Effects Accelerate Hot Carrier Relaxation but Slow Down Recombination in Metal Halide Perovskites

Nuclear Quantum Effects Accelerate Hot Carrier Relaxation but Slow Down Recombination in Metal Halide Perovskites

Inorganic semiconductors are composed of heavy elements whose vibrational motions are well described by classical mechanics. Heavy elements, such as Pb and I, support charge carriers in metal halide perovskites. Nevertheless, the soft structure and strong coupling between the organic and inorganic c...

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Bibliographic Details
Main Author: Yulong Liu (736976) (author)
Other Authors: Shiying Shen (7296863) (author), Oleg V. Prezhdo (1235424) (author), Run Long (1304349) (author), Wei-Hai Fang (1268982) (author)
Published: 2025
Subjects:
Biophysics
Medicine
Molecular Biology
Biotechnology
Science Policy
Physical Sciences not elsewhere classified
play important roles
inelastic scattering events
enhanced disorder makes
combining ab initio
intraband carrier relaxation
carrier relaxation processes
vibrational scattering responsible
support charge carriers
nuclear quantum effects
nqes influence structural
metal halide perovskites
light organic component
edge states plays
accelerate elastic electron
3 </ sub
vibrational dynamics
quantum zero
hot carriers
carrier recombination
well described
study offers
strong coupling
solar cells
soft structure
optoelectronic devices
opposite influences
heavy elements
electronic properties
detailed understanding
coherence loss
classical mechanics
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