Identifying Bottlenecks in the Photocatalytic Oxygen Evolution Reaction with Covalent Organic Frameworks

Covalent organic frameworks (COFs) have emerged as promising semiconducting materials for photocatalytic applications due to their large surface area, high crystallinity, and vast synthetic tunability. This is especially noticeable in the context of photocatalytic water splitting, where many COFs ha...

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محفوظ في:

التفاصيل البيبلوغرافية
المؤلف الرئيسي:	Stefan Trenker (21477936) (author)
مؤلفون آخرون:	Hugo A. Vignolo-Gonzalez (21477939) (author), Andrés Rodríguez-Camargo (12765804) (author), Liang Yao (823113) (author), Martijn A. Zwijnenburg (1301334) (author), Bettina V. Lotsch (1467520) (author)
منشور في:	2025
الموضوعات:	Biochemistry Medicine Molecular Biology Evolutionary Biology Computational Biology Environmental Sciences not elsewhere classified Chemical Sciences not elsewhere classified vast synthetic tunability using computational methods sandwich complex onto retained catalytic activity promising semiconducting materials large surface area hydrogen evolution half electrocatalytic tests indicate photocatalytic applications due photocatalytic water splitting sacrificial electron acceptor oxygen evolution cocatalyst ir ( iii careful control experiments control experiments subsequent photocatalytic water oxidation targeted cocatalyst evolve oxygen careful evaluation work demonstrates use heterogenization trace back reports focus pitfalls associated missing performance limited insight kinetic limitations identifying bottlenecks high crystallinity especially noticeable detailed role cof photocatalysts cobalt species bpy cof based cof anchored cp
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Identifying Bottlenecks in the Photocatalytic Oxygen Evolution Reaction with Covalent Organic Frameworks

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