Synthesis and Complexation Behavior of Well-Defined Polyester-Based Polyelectrolytes with Varying Charge Densities and Hydrophobicities

In this work, we describe the synthesis of polyester-based polyelectrolytes with varying charge densities and examine the complexation behavior of the corresponding polyelectrolyte complexes (PECs). The polyelectrolytes were prepared via ring-opening polymerization (ROP) of α-bromo-ε-caprolactone an...

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Bibliographic Details
Main Author:	Julian Engelhardt (10922613) (author)
Other Authors:	Louis C.P.M. de Smet (9127136) (author), Evelien Maaskant (10630719) (author), Jasper van der Gucht (831465) (author)
Published:	2025
Subjects:	Biophysics Biochemistry Biotechnology Marine Biology Plant Biology Space Science Environmental Sciences not elsewhere classified Chemical Sciences not elsewhere classified Physical Sciences not elsewhere classified prepared via ring critical salt concentration controllable material properties varying charge densities lowest charge densities polyelectrolyte mixtures show highest charge densities complex containing polyelectrolytes salt concentrations close developing novel polyester corresponding polyelectrolyte complexes complexes containing polyelectrolytes charge density polyelectrolyte complexation based polyelectrolytes highest csc subsequent postmodification strong tendency results using pecs ). opening polymerization nonmonotonic dependence nine combinations functionalized thiols findings pave findings imply field theory electrostatics play defined polyester based materials 100 %.
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Synthesis and Complexation Behavior of Well-Defined Polyester-Based Polyelectrolytes with Varying Charge Densities and Hydrophobicities

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