Three-Step Spin Crossover in a Pseudo-3D Hofmann-Type Complex Originating from Anisotropic Supramolecular Interactions

The development of multistep spin crossover materials is of considerable interest for molecular information processing and sensing applications and remains synthetically and mechanistically challenging. Herein, we present the first iron(II) two-dimensional Hofmann structure containing 1,2,4-triazole...

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Номзүйн дэлгэрэнгүй
Үндсэн зохиолч:	Xiaochun Li (143491) (author)
Бусад зохиолчид:	Nour-El-Islam Belmouri (21762681) (author), Mouhamadou Sy (2388802) (author), Mariusz Wolff (4807545) (author), Aurelian Rotaru (1613896) (author), Steven van Terwingen (10692886) (author), Dominik Maskowicz (14807802) (author), Miroslaw Sawczak (8124836) (author), Rafal Jendrzejewski (22772944) (author), Kamel Boukheddaden (1399912) (author), Yann Garcia (1727962) (author)
Хэвлэсэн:	2025
Нөхцлүүд:	Biophysics Biochemistry Molecular Biology Biotechnology Evolutionary Biology Chemical Sciences not elsewhere classified Physical Sciences not elsewhere classified step spin crossover sequential spin transition opens new avenues molecular information processing meophtrz )< sub including hydrogen bonding distinct transition steps dimensional structure assembled differential scanning calorimetry differential rigidity along cn )< sub anisotropic supramolecular framework type complex originating multiple intermolecular interactions anisotropic supramolecular interactions 2 </ sub supramolecular interactions interactions contribute complex exhibits n </ h </ e </ varied response tunable functionalities triazole derivatives sxrd reveals sxrd ), study highlights sensing applications remains synthetically ray diffraction raman spectroscopy optical microscopy methoxyphenyl )-< methanimine ). mechanistically challenging magnetic susceptibility likely driven like materials first iron crystallographic axes crystal x considerable interest >- 1 3d hofmann 2d hofmann
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Three-Step Spin Crossover in a Pseudo-3D Hofmann-Type Complex Originating from Anisotropic Supramolecular Interactions

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