Activation and Functionalization of the Uranyl Ion by Electrochemical Reduction

Activation and Functionalization of the Uranyl Ion by Electrochemical Reduction

Interconversion of the oxidation states of uranium enables separations and reactivity schemes involving this element and contributes to technologies for recycling of spent nuclear fuels. The redox behaviors of uranium species impact these processes, but use of electrochemical methods to drive reacti...

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Bibliographic Details
Main Author: Riddhi R. Golwankar (14822916) (author)
Other Authors: Małgorzata Z. Makoś (10492716) (author), Nathalia Cajiao (13176386) (author), Michael L. Neidig (1273662) (author), Allen G. Oliver (1314324) (author), Cynthia S. Day (1336956) (author), Victor W. Day (1312500) (author), Vassiliki-Alexandra Glezakou (1337457) (author), James D. Blakemore (1705078) (author)
Published: 2024
Subjects:
Computational Biology
Biological Sciences not elsewhere classified
Chemical Sciences not elsewhere classified
uranium enables separations
spent nuclear fuels
reactivity schemes involving
ray diffraction analysis
obtain molecular insights
multicomponent systems needed
molecular uranium complexes
molecular actinide species
joint computational studies
uranium species impact
methods commonly employed
chemical reactivity studies
promote stepwise functionalization
uranyl functionalization chemistry
electrochemical reduction interconversion
electrochemical methods
usually impact
uranyl ion
selective interconversion
chemical reductant
u –
taken together
structural data
spectroscopic findings
results suggest
redox behaviors
parallel electroanalytical
oxidation states
moderate electrophile
key reduced
key reactions
exogenous triphenylborane
driven reactions
drive reactions
disproportionation pathways
conventional requirement
changes associated
borylated products
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