Influence of Internal Interfaces on the Structure and Dynamics of IL-Based Electrolytes Confined in a Metal–Organic Framework

Hybrid solid-state electrolytes, which combine ionic liquids with metal–organic frameworks, offer a promising approach to enhancing the safety and energy density of next-generation batteries. A thorough understanding of the interplay between the solid and liquid phases in hybrid solid-state electrol...

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Bibliographic Details
Main Author:	Janis Hessling (21072185) (author)
Other Authors:	Leonard Dick (17311410) (author), Sophia Keil (21556573) (author), Vahideh Alizadeh (9243140) (author), Michael Ryan Hansen (1659685) (author), Barbara Kirchner (1385562) (author), Monika Schönhoff (1411822) (author)
Published:	2025
Subjects:	Biophysics Genetics Space Science Biological Sciences not elsewhere classified Chemical Sciences not elsewhere classified Physical Sciences not elsewhere classified fastest diffusing species combine ionic liquids 7 </ sup different ionic liquid li spin relaxation even make li sup >+</ sup generation battery applications although confinement within competitive interactions might ionic liquid cation increase li conductivity based electrolytes confined 8 hybrid system ionic liquid confined system battery electrolytes based electrolytes hybrid electrolytes liquid phases generation batteries competitive interaction 8 framework strong li local li enhance li elucidate li blocking li state electrolytes wall interactions thorough understanding study investigates state nmr state electrolyte results reveal raman spectroscopy promising approach overall decrease investigated using internal interfaces impedance spectroscopy hybrid solid energy density effective strategy chemical nature bulk electrolyte beneficial interactions anion clusters
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Influence of Internal Interfaces on the Structure and Dynamics of IL-Based Electrolytes Confined in a Metal–Organic Framework

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